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Characteristics of Metallic and Ionic Elements Concentration in PM10 at Guducsan in Busan

부산 구덕산 미세먼지의 금속성분 및 이온성분 농도 특성

  • Jeon, Byung-Il (Department of Environmental Engineering, Silla University)
  • Received : 2016.03.06
  • Accepted : 2016.03.28
  • Published : 2016.05.31

Abstract

This study investigates the characteristics of metallic and ionic elements concentration, concentration according to transport path, and factor analysis in $PM_{10}$ at Guducsan in Busan in the springtime of 2015. $PM_{10}$ concentration in Guducsan and Gwaebeopdong were $59.5{\pm}9.04{\mu}g/m^3$ and $87.5{\pm}20.2{\mu}g/m^3$, respectively. Contribution rate of water-soluble ions and secondary ion in $PM_{10}$ concentration in Guducsan were 37.0% and 27.8% respectively. [$NO_3{^-}/SO{_4}^{2-}$] ratio and contribution rate of sea salt of $PM_{10}$ in Guducsan and Gwaebeopdong were 0.91 and 1.12, 7.0% and 5.3%, respectively. The results of the backward trajectory analysis indicates that $PM_{10}$ concentration, total inorganic water-soluble ions and total secondary ions were high when the air parcels moved from Sandong region in China than non-Sandong and northen China to Busan area. The results of the factor analysis at Guducsan indicates that factor 1 was anthropogenic source effects such as automobile emissions and industrial combustion processes, factor 2 was marine sources such as sea salts from sea, and factor 3 was soil component sources.

Keywords

References

  1. Allen, G., Sioutas, C., Koutrakis, P., Reiss, R., Lurmann, F. W., Roberts, P. T., 1997, Evaluation of the TEOM method for measurement of ambient particulate mass in urban areas, Air & Waste Manage. Assoc., 47, 682-689. https://doi.org/10.1080/10473289.1997.10463923
  2. Arsene, C., Olariu, R. I., Mihalopoulos, N., 2007, Chemical composition of rainwater in the northeastern Romania, Iasi region (2003-2006), Atmos. Environ., 41, 9452-9467. https://doi.org/10.1016/j.atmosenv.2007.08.046
  3. Asman, W., Jaarsveld, H., 1991, A Variable-resolution transport model applied for NHX in Europe, Atmos. Environ., 24A, 445-464.
  4. Draxler, R. R., Rolph, G. D., 2013, HYSPLIT(HYbrid Single-Particle Lagrangian Integrated Trajectory) Model access via NOAA ARL READY Website (http://ready.arl.noaa.gov/HYSPLIT_traj.php).
  5. Ho, K. F., Lee, S. C., Chan, C. K., Yu, J. C., Chow, J. C., Yao, X. H., 2003, Characterization of chemical species in $PM_{2.5}$ and $PM_{10}$ aerosols in Hong Kong, Atmos. Environ., 37, 31-39. https://doi.org/10.1016/S1352-2310(02)00804-X
  6. Holland, H. D., 1978, The Chemistry of the Atmosphere and Ocean, John Wiley, Hoboken, New Jersey, USA.
  7. Jeon, B. I., 2015a, Meteorological relations and characteristics of fine particles at Guducksan in Busan, Sci. Inter., 24, 883-892.
  8. Jeon, B. I., 2015b, Weekday/weekend chemical characte-ristics of water-soluble components of $PM_{10}$ at Busan in springtime, Sci. Inter., 24, 785-792.
  9. Jeon, B. I., Hwang, Y. S., 2010, Chemical properties of the metallic composition and the mass concentration of $PM_{10}$ and $PM_{2.5}$ observed in Busan, Korea in springtime of 2006-2008, Kor. Earth Sci., 31(6), 234-245. https://doi.org/10.5467/JKESS.2010.31.3.234
  10. Jeon, B. I., Hwang, Y. S., 2014, Characteristics of metallic and ionic concentration in $PM_{10}$ and $PM_{2.5}$ in Busan, Sci. Inter., 23, 819-827.
  11. Jeon, B. I., Hwang, Y. S., Oh, K. J., 2010, Characteristics of metallic and ionic concentration in $PM_{10}$ at inland and seashore in Busan, Environ. Imp. Assess., 19, 323-333.
  12. Jung, C. H., Cho, Y. S., Hwang, S. M., Jung, Y. G., Ryu, J. C., Shin, D. S., 2007, Analysis of measurement error for PM-10 mass concentration by inter-comparison study, Kor. Atmos. Environ., 23(6), 689-698. https://doi.org/10.5572/KOSAE.2007.23.6.689
  13. Kim, K. Y., 2006, The Distribution of atmospheric sea-salt concentration Jeju Island, Master's thesis, Cheju National University, 62.
  14. Ko, H. J., Lim, E. H., Song, J. M., Kim, W. H., Kang, C. H., Lee, H. Y., Lee, C. K., 2015, Composition variation of atmospheric fine particulate matters in accordance with air mass transport pathways at background site of Korea in 2013, Kor. Atmos. Environ., 31(1), 15-27. https://doi.org/10.5572/KOSAE.2015.31.1.015
  15. Lee, S. B., Jung, D. S., Cho, E. K., Kim, H. A., Hwang, E. Y., Kang, C. H., 2011, Composition and pollution characteristics of $PM_{10}$ and $PM_{2.5}$ particles at Gosan site of Jeju Island in 2008, Anal. Sci. & Tech., 24(4), 310-318. https://doi.org/10.5806/AST.2011.24.4.310
  16. Li, K. C., Hwang, I. J., 2015, Characteristics of $PM_{2.5}$ in Gyeongsan using statistical analysis, Kor. Soc. Atmos. Environ., 31(6), 520-529. https://doi.org/10.5572/KOSAE.2015.31.6.520
  17. Logan, J. A., 1983, Nitrogen oxides in the troposphere : Global and regional budgets, Geophy. Rese., 88, 10785-10807. https://doi.org/10.1029/JC088iC15p10785
  18. Millero, F. J., Sohn, M. L., 1992, Chemical Oceanography, CRC Press, Boca Raton FL, 531.
  19. Oravisjarvi, K., Timonen, K. L., Wiikinkoski, T., Ruuskanen, A. R., Heinanen, K., Ruuskanen, J., 2003, Source contributions to $PM_{2.5}$ particles in the urban air of a town situated close to a steel works, Atmos. Environ., 31(8), 1013-1022.
  20. Park, G. H., Jeong, J. W., Cho, J. G., 2012, Evaluation of pollution characteristics and chemical composition of PM2.5 in the ambient air of Busan(III), The Annual Report of Busan Metro. city Insti. Heal. & Environ., 22(1), 142-159.
  21. Park, J. Y., Lim, H. J., 2006, Characteristics of water soluble ions in fine particles during the winter and spring in Daegu, Kor. Atmos. Environ., 22(5), 627-641.
  22. Sasaki, K., Sakamoto, K., 2005, Vertical differences in the composition of $PM_{10}$ and $PM_{2.5}$ in the urban atmosphere of Osaka, Japan Atmos. Environ., 39, 7240-7250. https://doi.org/10.1016/j.atmosenv.2005.09.004
  23. Willison, M. J., Clarke, A. G., Zeki, E. M., 1989, Chloride aerosols in central northern England, Atmos. Environ., 23(10), 2231-2239. https://doi.org/10.1016/0004-6981(89)90185-6
  24. Yao, X., Chan, C. K., Fang, M et al., 2002, The Water-soluble ionic composition of $PM_{2.5}$ in Shanghai and Beijing, China: 1-inorganic ions, Atmos. Environ., 36(26), 4223-4234. https://doi.org/10.1016/S1352-2310(02)00342-4
  25. Yoo, S. S., Jeon, J. S., Jung, K., Shin, E. S., Jung, B. J., Ryu, R. N., Woo, J. H., Sunwoo, Y., 2011, Analysis on air quality characteristics through air quality monitoring stations in urban background and high altitude in 2005-2006 in Seoul, Environ. Impact Assess., 49-59.
  26. Yoon, H. G., Kim, N. J., Kim, H. J., Jo, S. H., Lee, Y. M., Jeong, G., Kim, J. Y., Kim, M. Y., 2009, Characteristics of air quality at Gwanaksan, Proceeding of the 49th Meeting of KOSAE, 678-679.