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Source Analysis of Size Distribution and Density Estimation in PM2.5 -Part II

입경 분포 원인 분석 및 PM2.5 밀도 추정 -Part II

  • Bae, Min-Suk (Department of Environmental Engineering, Mokpo National University) ;
  • Park, Da-Jeong (Department of Environmental Engineering, Mokpo National University) ;
  • Lee, Jeonghoon (School of Mechanical Engineering, Korea University of Technology and Education) ;
  • Ahn, Joon-Young (National Institute of Environmental Research, Air Quality Research Division) ;
  • Lee, Yeong-Jae (National Institute of Environmental Research, Air Quality Research Division)
  • 배민석 (목포대학교 환경공학과) ;
  • 박다정 (목포대학교 환경공학과) ;
  • 이정훈 (한국기술교육대학교 기계공학부) ;
  • 안준영 (국립환경과학원 대기환경연구과) ;
  • 이영재 (국립환경과학원 대기환경연구과)
  • Received : 2016.01.17
  • Accepted : 2016.02.12
  • Published : 2016.04.30

Abstract

To characterize the features of particle apparent density, continuous measurements of particle number size distributions from optical particle sizer (OPS) and 24 hr integrated particle mass concentrations from filter based sampler were conducted at the National institute of environmental research NamBu Supersite (NNBS, $35.22^{\circ}N$, $126.84^{\circ}E$) in Gwangju for 16 days from Nov. 4 in 2014. Source apportionment model was carried out by applying Positive Matrix Factorization (PMF) to particle size distribution data. Three different distributions related to primary and secondary sources were investigated by the diurnal patterns of identified factors. Density estimated by gaussian model has been calculated as $1.69g/cm^3$ with 95% confidence bounds ($1.57{\sim}1.81g/cm^3$).

Keywords

References

  1. Abegglen, M., L. Durdina, B.T. Brem, J. Wang, T. Rindlisbacher, J.C. Corbin, U. Lohmann, and B. Sierau (2015) Effective density and mass-mobility exponents of particulate matter in aircraft turbine exhaust : Dependence on engine thrust and particle size, J. Aerosol Sci., 88, 135-147. https://doi.org/10.1016/j.jaerosci.2015.06.003
  2. Bae, M.S., S.S. Park, and Y.J. Kim (2013) Characteristics of carbonaceous aerosols measured at Gosan- Based on analysis of thermal distribution by carbon analyzer and organic compounds by GCMS, J. Korean Soc. Atmos. Environ., 29(6), 722-733. (in Korean with English Abstract) https://doi.org/10.5572/KOSAE.2013.29.6.722
  3. Cassee, F.R., M.E. Heroux, M.E. Gerlofs-Nijland, and F.J. Kelly (2013) Particulate matter beyond mass: recent health evidence on the role of fractions, chemical constituents and sources of emission, Inhal. Toxicol., 25(14), 802-812. https://doi.org/10.3109/08958378.2013.850127
  4. Castellini, S., B. Moroni, and D. Cappelletti (2014) PMetro: Measurement of urban aerosols on a mobile platform, Meas., 49(1), 99-106. https://doi.org/10.1016/j.measurement.2013.11.045
  5. Cho, I.H., D.J. Park, and M.S. Bae (2015) Time Resolved Analysis of Water Soluble Organic Carbon by Aerosolinto-Mist System, J. Korean Soc. Atmos. Environ., 31(6), 497-507. (in Korean with English Abstract) https://doi.org/10.5572/KOSAE.2015.31.6.497
  6. Cooper, G., J. Foster, L. Galbraith, S. Jain, A. Neukermans, and B. Ormond (2014) Preliminary results for salt aerosol production intended for marine cloud brightening, using effervescent spray atomization, Phil. Trans. R. Soc. A, 372, 20140055. https://doi.org/10.1098/rsta.2014.0055
  7. DeCarlo, P.F., J.G. Slowik, D.R. Worsnop, P. Davidovits, and J.L. Jimenez (2004) Particle morphology and density characterization by combined mobility and aerodynamic diameter measurements. Part 1 Theory, Aerosol Sci. Technol., 38(12), 1185-1205. https://doi.org/10.1080/027868290903907
  8. Franck, U., S. Odeh, A. Wiedensohler, B. Wehner, and O. Herbarth (2011) The effect of particle size on cardiovascular disorders: the smaller the worse, Sci. Total Environ., 409(20), 4217-4221. https://doi.org/10.1016/j.scitotenv.2011.05.049
  9. Ham, W.A. and M.J. Kleeman (2011) Size-resolved source apportionment of carbonaceous particulate matter in urban and rural sites in central California, Atmos. Environ., 45(24), 3988-3995. https://doi.org/10.1016/j.atmosenv.2011.04.063
  10. Hand, J.L., S.M. Kreidenweis, N. Kreisberg, S. Hering, M. Stolzenburg, W. Dick, and P.H. McMurry (2002) Comparisons of aerosol properties measured byimpactors and light scattering from individual particles: refractive index, number and volume concentrations, and size distributions, Atmos. Environ., 36(11), 1853-1861. https://doi.org/10.1016/S1352-2310(02)00103-6
  11. Hasheminassab, S., P. Pakbin, R.J. Delfino, J.J. Schauer, and C. Sioutas (2014) Diurnal and seasonal trends in the apparent density of ambient fine and coarse particles in Los Angeles, Environ. Pollut., 187, 1-9. https://doi.org/10.1016/j.envpol.2013.12.015
  12. Hu, M., J. Peng, K. Sun, D. Yue, S. Guo, A. Wiedensohler, and Z. Wu (2012) Estimation of size-resolved ambient particle density based on the measurement of aerosol number, mass, and chemical size distributions in the Winter in Beijing, Environ. Sci. Technol., 46(18), 9941-9947. https://doi.org/10.1021/es204073t
  13. Hussein, T., C. Johansson, H. Karlsson, and H.C. Hansson (2008) Factors affecting nontailpipe aerosol particle emissions from paved roads: on-road measurements in Stockholm, Sweden, Atmos. Environ., 42(4), 688-702. https://doi.org/10.1016/j.atmosenv.2007.09.064
  14. Jeong, Y.J. and I.J. Hwang (2015) Source Apportionment of $PM_{2.5}$ in Gyeongsan Using the PMF Model, J. Korean Soc. Atmos. Environ., 31(6), 508-519. (in Korean with English Abstract) https://doi.org/10.5572/KOSAE.2015.31.6.508
  15. Kraus, U., S. Breitner, J. Schnelle-Kreis, J. Cyrys, T. Lanki, R. Ruckerl, A. Schneider, I. Bruske, J.W. Gu, R. Devlin, H.E. Wichmann, R. Zimmermann, and A. Peters (2011) Particle-associated organic compounds and symptoms in myocardial infarction survivors, Inhal. Toxicol., 23(7), 431-447. https://doi.org/10.3109/08958378.2011.580471
  16. Lee, J., B. Jeong, D.J. Park, and M.S. Bae (2015a) A Study of Black Carbon Measurement in Metropolitan Area and Suburban Area of the Korean Peninsula Performed during Pre KORea-US Air Quality Study (KORUS-AQ) Campaign, J. Korean Soc. Atmos. Environ., 31(5), 472-481. (in Korean with English Abstract) https://doi.org/10.5572/KOSAE.2015.31.5.472
  17. Lee, T., J. Choi, G. Lee, J. Ahn, J.S. Park, S.A. Atwood, M. Schurman, Y. Choi, Y. Chung, and J.L. Collett Jr, (2015b) Characterization of aerosol composition, concentrations, and sources at Baengnyeong Island, Korea using an aerosol mass spectrometer, Atmos. Environ., 120, 297-306. https://doi.org/10.1016/j.atmosenv.2015.08.038
  18. Lee, Y., M. Park, S. Jung, S. Kim, M. Jo, I. Song, Y. Lyu, Y. Lim, J. Kim, H. Jung, S. Lee, W. Choi, J. Ahn, M. Lee, H. Kang, S. Park, S. Seo, D. Jung, J. Hyun, J. Park, T. Hwang, Y. Hong, J. Hong, and H. Shin (2015) Characteristics of Particulate Carbon in the Ambient Air in the Korean Peninsula, J. Korean Soc. Atmos. Environ., 31(4), 330-344. (in Korean with English Abstract) https://doi.org/10.5572/KOSAE.2015.31.4.330
  19. Levy, M.E., R.Y. Zhang, A.F. Khalizov, J. Zheng, D.R. Collins, C.R. Glen, Y. Wang, X.Y. Yu, W. Luke, J.T. Jayne, and E. Olaguer (2013) Measurements of submicron aerosols in Houston, Texas during the 2009 SHARP field campaign. J. Geophys. Res. D: Atmos., 118, 10518-10534. https://doi.org/10.1002/jgrd.50785
  20. Liu, Z., B. Hu, D. Ji, Y. Wang, M. Wang, and Y. Wang (2015) Diurnal and seasonal variation of the $PM_{2.5}$ apparent particle density in Beijing, China, Atmos. Environ., 120, 328-338. https://doi.org/10.1016/j.atmosenv.2015.09.005
  21. Liu, Z., B. Hu, Q. Liu, Y. Sun, and Y.S. Wang (2014) Source apportionment of urban fine particle number concentration during summertime in Beijing, Atmos. Environ., 96, 359-369. https://doi.org/10.1016/j.atmosenv.2014.06.055
  22. McMurry, P.H., X. Wang, K. Park, and K. Ehara (2002) The relationship between mass and mobility for atmospheric particles: a new technique for measuring particle density, Aerosol Sci. Technol., 36(2), 227-238. https://doi.org/10.1080/027868202753504083
  23. Paatero, P. (1997) Least squares formulation of robust nonnegative factor analysis, Chemom. Intell. Lab. Syst., 37(1), 23-35. https://doi.org/10.1016/S0169-7439(96)00044-5
  24. Park, D.J., J.Y. Ahn, H.J. Shin, and M.S. Bae (2014) Characteristics of $PM_{2.5}$ Carbonaceous Aerosol using PILSTOC and GC/MS-TD in Seoul, J. Korean Soc. Atmos. Environ., 30(5), 461-476. (in Korean with English Abstract) https://doi.org/10.5572/KOSAE.2014.30.5.461
  25. Park, D.J., K.Y. Lee, K. Park, and M.S. Bae (2016) Diurnal Size Distributions of Black Carbon by comparison of Optical Particulate Measurements - Part I, J. Korean Soc. Atmos. Environ., 32(1), 1-8. (in Korean with English Abstract) https://doi.org/10.5572/KOSAE.2016.32.1.001
  26. Pitz, M., O. Schmid, J. Heinrich, W. Birmili, J.R. Maguhn, R. Zimmermann, H.E. Wichmann, A. Peters, and J. Cyrys (2008) Seasonal and diurnal variation of $PM_{2.5}$ apparent particle density in urban air in Augsburg, Germany, Environ. Sci. Technol., 42(14), 5087-5093. https://doi.org/10.1021/es7028735
  27. Schmid, O., E. Karg, D.E. Hagen, P.D. Whitefield, and G.A. Ferron (2007) On the effective density of non-spherical particles as derived from combined measurements of aerodynamic and mobility equivalent size, J. Aerosol Sci., 38(4), 431-443. https://doi.org/10.1016/j.jaerosci.2007.01.002
  28. Xu, B., Y. Wu, Z. Lin, and Z. Chen (2014) Investigation of Air Humidity Affecting Filtration Efficiency and Pressure Drop of Vehicle Cabin Air Filters, Aerosol Air Qual. Res., 14(3), 1066-1073. https://doi.org/10.4209/aaqr.2013.06.0204
  29. Yin, Z., X. Ye, S. Jiang, Y. Tao, Y. Shi, X. Yang, and J. Chen (2015) Size-resolved effective density of urban aerosols in Shanghai, Atmos. Environ., 100, 133-140. https://doi.org/10.1016/j.atmosenv.2014.10.055
  30. Zhang, Y., R.J. Sheesley, M.S. Bae, and J.J. Schauer (2009) Sensitivity of a molecular marker based positive matrix factorization model to the number of receptor observations, Atmos. Environ., 43(32), 4951-4958. https://doi.org/10.1016/j.atmosenv.2009.07.009

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