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Transition temperatures and upper critical fields of NbN thin films fabricated at room temperature

  • Hwang, T.J. (Yeungnam University) ;
  • Kim, D.H. (Yeungnam University)
  • Received : 2015.09.01
  • Accepted : 2015.09.22
  • Published : 2015.09.30

Abstract

NbN thin films were deposited on thermally oxidized Si substrate at room temperature by using reactive magnetron sputtering in an $Ar-N_2$ gas mixture. Total sputtering gas pressure was fixed while varying $N_2$ flow rate from 1.4 sccm to 2.9 sccm. X-ray diffraction pattern analysis revealed dominant NbN(200) orientation in the low $N_2$ flow rate but emerging of (111) orientation with diminishing (200) orientation at higher flow rate. The dependences of the superconducting properties on the $N_2$ gas flow rate were investigated. All the NbN thin films showed a small negative temperature coefficient of resistance with resistivity ratio between 300 K and 20 K in the range from 0.98 to 0.89 as the $N_2$ flow rate is increased. Transition temperature showed non-monotonic dependence on $N_2$ flow rate reaching as high as 11.12 K determined by the mid-point temperature of the transition with transition width of 0.3 K. On the other hand, the upper critical field showed roughly linear increase with $N_2$ flow rate up to 2.7 sccm. The highest upper critical field extrapolated to 0 K was 17.4 T with corresponding coherence length of 4.3 nm. Our results are discussed with the granular nature of NbN thin films.

Keywords

References

  1. J. R. Gavaler, J. K. Hulm, M. A. Janocko and C. K. Jones, "Preparation and Superconducting Properties of Thin Films of Transition Metal Interstitial Compounds," J. Vac. Sci. Technol., vol. 6, pp. 177-179, 1969. https://doi.org/10.1116/1.1492653
  2. J. Talvacchio and A. I. Braginski, "Tunnel junctions fabricated from coherent NbN/MgO/NbN and NbN/$Al_2O_3$/NbN structures," IEEE Trans. Magn., vol. 23, pp. 859-862, 1987. https://doi.org/10.1109/TMAG.1987.1064985
  3. J. Tyan and J. T. Lue, "Grain boundary scattering in the normal state resistivity of superconducting NbN thin films," J. Appl. Phys., vol. 75, pp. 325-331, 1994. https://doi.org/10.1063/1.355853
  4. Y. Pellan, G. Dousselin and J. Pinel, "Temperature and Magetic Field Dependence of NbN Film Resistivity: 3D Weak Localization Effects," J. Low Temp. Phys., vol. 78, pp. 63-77, 1990. https://doi.org/10.1007/BF00682110
  5. Y. Ufuktepe, A. H. Farba, S. I. Kimura, T. Hajiri, K. Imura, M. A. Mamun, F. Karadag, A. A. Elmustafa and H. E. Elsayed-Ali, "Supercnducting niobium nitride thin films by reactive pulsed laser deposition," Thin Solid Films, vol. 545, pp. 601-607, 2013. https://doi.org/10.1016/j.tsf.2013.08.051
  6. M. Ziegler, L. Fritzsch, J. Day, S. Linzen, S. Anders, J. Toussaint, and H. Meyer, "Superconducting niobium nitride thin films deposited by metal organic plasma-enhanced atomic layer deposition," Supercond. Sci. Technol., vol. 26, pp. 025008, 2013. https://doi.org/10.1088/0953-2048/26/2/025008
  7. A. Shoji, S. Kiryu and S. Kohjiro, "Superconducting properties and normal-state resistivity of single-crystal NbN films prepared by a reactive rf-magnetron method," Appl. Phys. Lett., vol. 60, pp. 1624-1626, 1992. https://doi.org/10.1063/1.107220
  8. J.-C. Villegier, N. Hadack, S. Monso, B. Delaet, A. Roussy, P. Febvre, G. Lamura and J.-Y. Laval, "NbN multilayer technology on R-plane sapphire," IEEE Trans. Appl. Superconduct., vol. 11, pp. 68-71, 2001. https://doi.org/10.1109/77.919286
  9. J. J. Zhang, X. Su, L. Zhang, L. Zheng, X. F. Wang and L. You, "Improvement of the superconducting properties of NbN thin film on single-crystal silicon substrate by using a TiN buffer layer," Supercond. Sci. Technol., vol. 26, pp. 045010, 2013. https://doi.org/10.1088/0953-2048/26/4/045010
  10. S. P. Chockalingam, M. Chand, J. Jesudasan, V. Tripathi and P. Raychaudhuri, "Superconducting properties and Hall effect of epitaxial NbN thin films," Phys. Rev. B., vol. 77, pp. 214503, 2008. https://doi.org/10.1103/PhysRevB.77.214503
  11. C. S. Menon and V. S. Pankajakshan, "Electrical conductivity and transition temperature of NbN thin films," Bull. Mater. Soc., vol. 9, pp.187-191, 1987. https://doi.org/10.1007/BF02744267

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