DOI QR코드

DOI QR Code

Evaluation of Adsorption Characteristics of Radioactive Iodine (I-131) for Various Materials of Granular Activated Carbon (GAC)

입상활성탄 재질별 방사성 핵종(I-131) 흡착 특성 평가

  • 박홍기 (부산광역시 상수도사업본부 수질연구소) ;
  • 손희종 (부산광역시 상수도사업본부 수질연구소) ;
  • 염훈식 (부산광역시 상수도사업본부 수질연구소) ;
  • 김영진 (부산광역시 상수도사업본부 수질연구소) ;
  • 최진택 (부산광역시 상수도사업본부 수질연구소) ;
  • 류동춘 (부산광역시 상수도사업본부 수질연구소)
  • Received : 2015.04.02
  • Accepted : 2015.09.09
  • Published : 2015.09.30

Abstract

This research was performed by means of several different virgin granular activated carbons (GAC) made of each coal, coconut and wood, and the GACs were investigated for an adsorption performance of iodine-131 in a continuous adsorption column. Breakthrough behavior was investigated that the breakthrough points of the virgin two coals-, coconut- and wood-based GACs were observed as bed volume (BV) 7080, BV 5640, BV 5064 and BV 3192, respectively. The experimental results of adsorption capacity (X/M) for iodine-127 showed that two coal- based GACs were highest (208.6 and $139.1{\mu}g/g$), the coconut-based GAC was intermediate ($86.5{\mu}g/g$) and the wood-based GAC was lowest ($54.5{\mu}g/g$). The X/M of the coal-based GACs was 2~4 times higher than the X/M of the coconut-based and wood-based GACs.

Keywords

References

  1. Gafvert, T., Ellmark, C., Holm, E., 2002, Removal of radionuclides at a waterworks, J. Environ. Radioactivity, 63(2), 105-115. https://doi.org/10.1016/S0265-931X(02)00020-6
  2. Goossens, R., Delville, A., Genot, J., Halleux, R., Masschelein, W. J., 1989, Removal of the typical isotopes of the chernobyl fall-out by conventional water treatment, Water. Res., 23(6), 693-697. https://doi.org/10.1016/0043-1354(89)90201-7
  3. Huang, C. P., 1978, Chemical interactions between inorganics and activated carbon, In: Carbon Adsorption Handbook, Cheremisinoff, P. N. and Ellerbusch, F., (Eds) Ann Arbor Science Publishers, Inc, Ann Arbor, Miami, 281-329.
  4. Ikemoto, T., Magara, Y., 2011, Measures against impacts of nuclear disaster on drinking water supply systems in Japan, Water Practice and Technology, 6(4), doi:10.2166/wpt.2011.078.
  5. Jeong, G., Lee, K., Kim, B., Lee, S., Lee, J., Koo, A., 2014, Study on removal of artificial radionuclide (I-131) water, J. Kor. Soc. Environ. Eng., 36(11), 747-752. https://doi.org/10.4491/KSEE.2014.36.11.747
  6. Kosaka, K., Asami, M., Kobashigawa, N., Ohkubo, K., 2012, Removal of radioactive iodine and cesiym in water purification processes after an explosion at a nuclear power plant due to the great japan Earthquake, Water. Res., 46, 4397-4404. https://doi.org/10.1016/j.watres.2012.05.055
  7. Morita, T., Niwa, K., Fujimoto, K., Kasai, H., Yamada, H., 2010, Detection and activity of iodine-131 in brown algae collected in the Japanese coastal areas, Sci. Total Environ., 408, 3443-3447. https://doi.org/10.1016/j.scitotenv.2010.04.001
  8. Siddiqui, M., Zhai, W., Amy, G., Mysore, C., 1996, Bromate ion removal by activated carbon, Water Res., 30, 1651-1660. https://doi.org/10.1016/0043-1354(96)00070-X
  9. Son, H. J., Jung, J. M., Hwang, Y. D., Roh, J. S., Yoo, P. J., 2008, Effects of activated carbon types and service life on adsorption of tetracycline antibiotic compounds in GAC process, J. Kor. Soc. Environ. Eng., 30(9), 925-932.
  10. Son, H. J., Yeom, H. S., Ryu, D. C., Jang, S. H., Son, H. S., 2014, Characteristics of adsorption and biode-gradation of tetracycline antibiotics by granular activated carbon and biofiltration process, J. Environ. Sci. Intl., 23(3), 379-386. https://doi.org/10.5322/JESI.2014.23.3.379
  11. Summers, R. S., Fuchs, F., Sontheimer, H., 1988, The fate and removal of radioactive iodine in the aquatic environment, In: Aquatic Humic Substances, 623-636.
  12. Tagami, K., Uchida, S., 2011, Can we remove iodine-131 from tap water in Japan by boiling? -experimental testing in response to the Fukushima Daiichi Nuclear Power Plant accident, Chemosphere, 84, 1282-1284. https://doi.org/10.1016/j.chemosphere.2011.05.050