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Spatial Distributions of On-road Ultrafine Particle Number Concentration on Naebu Express Way in Seoul during Winter Season

겨울철 서울 내부순환로 도로상 초미세입자 오염의 공간분포 특징

  • Woo, Daekwang (Center for Environment, Health and Welfare Research, Korea Institute of Science and Technology) ;
  • Lee, Seung-Bok (Center for Environment, Health and Welfare Research, Korea Institute of Science and Technology) ;
  • Lee, Seung Jae (Center for Environment, Health and Welfare Research, Korea Institute of Science and Technology) ;
  • Kim, Jin Young (Center for Environment, Health and Welfare Research, Korea Institute of Science and Technology) ;
  • Jin, Hyun Chul (Center for Environment, Health and Welfare Research, Korea Institute of Science and Technology) ;
  • Kim, Taesung (Department of Mechanical Engineering, Sungkyunkwan University) ;
  • Bae, Gwi-Nam (Center for Environment, Health and Welfare Research, Korea Institute of Science and Technology)
  • 우대광 (한국과학기술연구원 환경복지연구단) ;
  • 이승복 (한국과학기술연구원 환경복지연구단) ;
  • 이승재 (한국과학기술연구원 환경복지연구단) ;
  • 김진영 (한국과학기술연구원 환경복지연구단) ;
  • 진현철 (한국과학기술연구원 환경복지연구단) ;
  • 김태성 (성균관대학교 기계공학부) ;
  • 배귀남 (한국과학기술연구원 환경복지연구단)
  • Received : 2012.09.08
  • Accepted : 2012.12.04
  • Published : 2013.02.28

Abstract

To understand the traffic emissions with high temporal and spatial resolutions on road, a mobile laboratory was developed. The objective of this study is to characterize on-road air pollution on Naebu express way surrounding the northern area of Seoul, Korea. We measured the number concentration of ultrafine particles larger than 5 nm and particle size distribution using a condensation particle counter and a fast mobility particle sizer, respectively on 3, 7, and 8 December 2009. The average ultrafine particle number concentration on the Naebu express way excluding tunnels was 126,000 particles/$cm^3$ and 4.2 times higher than that on internal road at Korea Institute of Science and Technology in Seoul, and more than twice higher than that measured on and at the arterial roads of Seoul in previous studies. The maximum ultrafine particle number concentration was observed at the tunnel sections. It was 232,000 particles/$cm^3$ and 1.8 times higher than average ultrafine particle number concentration for the other sections on Naebu express way. The ultrafine particle number concentration on the wider roads with higher traffic volume along the Han River was similar to that in the residential section, probably because of enhanced dilution effect in widely open environment. The size distribution of particles on the Naebu express way was highly fluctuated for a short duration. Ultrafine particles measured at the tunnel showed a bimodal size distribution with mode diameters of ~10 nm and ~50 nm. At the Han riverside section, ~10 nm particles appeared significantly compared with size distribution at the tunnel. This on-road measurement approach can be utilized to manage vehicle-related air pollution in urban area.

Keywords

References

  1. Andre, M., R. Joumard, R. Vidon, P. Tassel, and P. Perret (2006) Real-world European driving cycles, for measuring pollutant emissions from high- and low-powered cars, Atmos. Environ., 40(31), 5944-5953. https://doi.org/10.1016/j.atmosenv.2005.12.057
  2. Attfiled, M.D., P.L. Schleiff, J.H. Lubin, A. Blair, P.A. Stewart, R. Vermeulen, J.B. Coble, and D.T. Silverman (2012) The diesel exhaust in miners study: A cohort mortality study with emphasis on lung cancer, J. Natl. Cancer Inst., 104(11), 869-883. https://doi.org/10.1093/jnci/djs035
  3. Bae, G.-N., S. Huh, S.-B. Lee, M. An, D. Park, and J. Hwang (2007) Ultrafine particle pollution level at the roadside of Seoul in spring, Part. Aerosol Res., 3(1), 29-40. (in Korean with English abstract)
  4. Bae, G.-N., S.J. Lee, H.-C. Jin, S.-B. Lee, S.-J. Woo, S.-H. Lee, J.-Y. Kim, and D.-C. Shin (2009) Development of a mobile emission laboratory for evaluation of air pollution nearby traffic, 2009 Fall Conference of the Korean Soc. for Atmos. Environ., 231-232. (in Korean with English abstract)
  5. Cocker III, D.R., S.D. Shah, K. Johnson, and J.M. Norbeck (2004a) Development and application of a mobile laboratory for measuring emissions from diesel engines. 1. Regulated gaseous emissions, Environ. Sci. Technol., 38(7), 2182-2189. https://doi.org/10.1021/es034888d
  6. Cocker III, D.R., S.D. Shah, K. Johnson, X. Zhum, J.W. Miller, and J.M. Norbeck (2004b) Development and application of a mobile laboratory for measuring emissions from diesel engines. 2. Sampling for toxics and particulate matter, Environ. Sci. Technol., 38(24), 6809-6816. https://doi.org/10.1021/es049784x
  7. Hagler, G.S., E.D. Thoma, and R.W. Baldauf (2010) High-resolution mobile monitoring of carbon monoxide and ultrafine particle concentrations in a near-road environment, J. Air & Waste Manage. Assoc., 60(3), 328-336. https://doi.org/10.3155/1047-3289.60.3.328
  8. Han, S., K.-H. Won, K.-W. Jang, Y.-M. Son, J.-S. Kim, J.-H. Hong, and Y.-W. Jung (2007) Development and application of real-time measurement system of silt loading for estimating the emission factor of resuspended dust from paved road, Korean J. of Atmos. Environ., 23(5), 596-611. https://doi.org/10.5572/KOSAE.2007.23.5.596
  9. Joumard, R., M. Andre, R. Vidon, P. Tassel, and C. Pruvost (2000) Influence of driving cycles on unit emissions from passenger cars, Atmos. Environ., 34(27), 4621-4628. https://doi.org/10.1016/S1352-2310(00)00118-7
  10. Kim, M.-H., S.-G. Park, and S.-O. Baek (2002) Characteristics of atmospheric concentrations of volatile organic compounds at a heavy-traffic site in a large urban area, Korean J. of Atmos. Environ., 18(2), 113-126. (in Korean with English abstract).
  11. Kittelson, D., J. Johnson, W. Watts, Q. Wei, M. Drayton, D. Paulsen, and N. Bukowiecki (2000) Diesel aerosol sampling in the atmosphere, Society of Automotive Engineers Technical Paper Series, No. 2000-01- 2212, Warrendale, PA, USA.
  12. Kittelson, D., W.F. Watts, and J.P. Johnson (2004) Nanoparticle emissions on Minnesota highways, Atmos. Environ., 38(1), 9-19. https://doi.org/10.1016/j.atmosenv.2003.09.037
  13. Kwon, O.-Y. and Y.S. An (2006) Temporal and spatial distributions of $PM_10$, $NO_x$ and $O_3$ around the road, Korean J. of Atmos. Environ., 22(4), 440-450. (in Korean with English abstract)
  14. Lee, J., M. Jung, Y. Jeong, and K. Cha (2008) Analysis of diesel nano-particle characteristics for different vehicle test mode in diesel passenger vehicle, Trans. of KSAE, 16(1), 114-120. (in Korean with English abstract)
  15. Lee, S.-B. and G.-N. Bae (2010) Characteristics of air pollution at a junction area contaminated with vehicle emissions, Trans. of KSAE, 18(4), 48-53. (in Korean with English abstract)
  16. Lee, S.-B., D.-H. Lee, S.J. Lee, H.-C. Jin, and G.-N. Bae (2011) Characteristics of spatial distribution of ultrafine particle number concentration on the roads of Nowon-gu, Seoul, Part. Aerosol Res., 7(1), 21-30. (in Korean with English abstract)
  17. Lee, Y., C. Cho, G. Kim, J.Y. Jung, I. Song, and H. Jung (2008) On-road measurement of exhaust emissions by remote sensing device, Proceeding of Korean Society of Automotive Engineers 30th Anniversary Conference, 416-420. (in Korean with English abstract)
  18. Mills, N.L., H. Tornqvist, M.C. Gonzalez, E. Vink, S.D. Robinson, S. Soderberg, N.A. Boon, K. Donaldson, T. Sandström, A. Blomberg, and D.E. Newby (2007) Ischemic and thrombotic effects of dilute dieselexhaust inhalation in men with coronary heart disease, N. Engl. J. Med., 357(11), 1075-1082. https://doi.org/10.1056/NEJMoa066314
  19. Park, B.-E., S.-B. Lee, D.-H. Lee, S.J. Lee, D.-K. Woo, J.-H. Choi, H.-C. Jin, G.-N. Bae, and S.-T. Yun (2012) Spatial distribution of air pollution level inside roadway tunnels in urban area, Part. Aerosol Res., 8(1), 17-28. (in Korean with English abstract)
  20. Park, S.-K., S.-D. Kim, and J.-H. Kim (1998) A study of concentration prediction of automobile air pollutant near the highway, Korean J. of Atmos. Environ., 14(6), 607-620. (in Korean with English abstract)
  21. Park, Y.-H., J.-C. Kim, S.-I. Kwon, T.-W. Lee, and J.-T. Lee (2005) A study on the improvement in-use vehicle inspection & maintenance program by RSD (remote sensing detector), Proceeding of Korean Society of Automotive Engineers 2005 Fall Conference, 159-164. (in Korean with English abstract)
  22. Samet, J.M., S. Zeger, F. Dominici, and F.C. Curreiero (2000) The National Morbidity, Mortality, and Air Pollution Study (NMMAPS): Part 2. Morbidity and Mortality from Air Pollution in the United States, Health Effects Institutes.
  23. Schneider, J., U. Kirchner, S. Borrmann, R. Vogt, and V. Scheer (2008) In situ measurements of particle number concentration, chemically resolved size distributions and black carbon content of traffic-related emissions on German motorways, rural roads and in city traffic, Atmos. Environ., 42(18), 4257-4268. https://doi.org/10.1016/j.atmosenv.2008.01.014
  24. Silverman, D.T., C.M. Samanic, J.H. Lubin, A.E. Blair, P.A. Stewart, R. Vermeulen, J.B. Coble, N. Rothman, P.L. Schleiff, W.D. Travis, R.G. Ziegler, S. Wacholder, and M.D. Attfield (2012) The diesel exhaust in miners study: A nested case-control study of lung cancer and diesel exhaust, J. Natl. Cancer Inst., 104 (11), 855-868. https://doi.org/10.1093/jnci/djs034
  25. Son, B.S. (1999) Development of strategies and methods for improving the mobility, accessibility, traffic safety and capacity of Naebu express way in Seoul (99-07), Seoul Development Institute, Seoul.
  26. Westerdahl, D., X. Wang, X. Pan, and K.M. Zhang (2009) Characterization of on-road vehicle emission factors and microenvironmental air quality in Beijing, China, Atmos. Environ., 43(3), 697-705. https://doi.org/10.1016/j.atmosenv.2008.09.042
  27. Woo, D., S.-B. Lee, G.-N. Bae, and T. Kim (2008) Comparison of ultrafine particles monitored at a roadside using an SMPS and a TR-DMPS, Korean J. of Atmos. Environ., 24(4), 404-414. (in Korean with English abstract) https://doi.org/10.5572/KOSAE.2008.24.4.404
  28. Zhu, Y., W.C. Hinds, S. Kim, and C. Sioutas (2002) Concentration and size distributions of ultrafine particles near a major highway, J. Air & Waste Manag. Assoc., 52(9), 1032-1042. https://doi.org/10.1080/10473289.2002.10470842