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Tb3+ and Ce3+ Intercalated Laponite Powder: The Influence of Ce3+ Ions on Thermal Stability and Optical Properties of Tb3+ Intercalated Laponite

  • Lee, Han-Na (Department of Chemistry and Institute of Basic Sciences, College of Advanced Sciences, Dankook University) ;
  • Kim, You-Hyuk (Department of Chemistry and Institute of Basic Sciences, College of Advanced Sciences, Dankook University)
  • Received : 2011.01.11
  • Accepted : 2011.02.17
  • Published : 2011.04.20

Abstract

Laponite samples intercalated with $Tb^{3+}$ or $Tb^{3+},Ce^{3+}$ ions were prepared by exchange of Na+ ions in interlayers with $Tb^{3+}$ or $Ce^{3+}$ ions. Strong green and weak blue emissions under vacuum ultraviolet (VUV) excitation (${\lambda}$ = 158 nm) were observed due to the $^5D_4{\rightarrow}^7F_J$ and $^5D_3{\rightarrow}^7F_J$ emission lines, respectively. $Tb^{3+}$ ions in an interlayer of laponite mainly existed in ion pairs or clusters, as evidenced by the concentration-dependent luminescence of the $Tb^{3+}$ ions on the relative intensities of the $^5D_3{\rightarrow}^7F_J$ and the $^5D_4{\rightarrow}^7F_J$ emission lines, due to the action of a cross-relaxation process. The addition of $Ce^{3+}$ ions increased the thermal stability of $Tb^{3+}$ intercalated laponite up to $650^{\circ}C$ and quenched the $^5D_3{\rightarrow}^7F_J$ emission lines, probably by promoting the formation of $Tb^{3+}$ ion pairs at relatively low $Tb^{3+}$ concentrations.

Keywords

References

  1. Laird, D. A. Applied Clay Sci. 2006, 34, 74. https://doi.org/10.1016/j.clay.2006.01.009
  2. Shichi, T.; Takagi, K. J. Photochem & Photobio. C: Photochem. Rev. 2000, 30, 113.
  3. Gerstl, Z.; Nasser, A.; Mingelgrin, U. J. Agric. Food Chem. 1998, 46, 3797. https://doi.org/10.1021/jf980185h
  4. Ohtsuka, K.; Hayashi, Y. Chem. Mater. 2001, 13, 704. https://doi.org/10.1021/cm0004329
  5. Greaves, R. C.; Bond, S. P.; McWhinnie, W. R. Polyhedron 1995,14, 3635. https://doi.org/10.1016/0277-5387(95)00158-O
  6. Avery, R. G.; Ramsay, J. D. F. J. Colloid Interface Sci. 1986, 109,448. https://doi.org/10.1016/0021-9797(86)90322-X
  7. Yen, W. M.; Shionoya, S.; Yamamoto, H., Eds.; Phosphor Handbook, 2nd ed.; CRC: Boca Raton, FL, 2007.
  8. Kim, P.-R.; Son, D.-M.; Lee, H.-N.; Kim, Y. J. Kor. Cryst. Growth & Cryst. Tech. 2009, 19, 196.
  9. Tronto, J.; Ribeiro, S. J. L.; Valim, J. B.; Gonçalves, R. R. Mat. Chem. & Phys. 2009, 113, 71. https://doi.org/10.1016/j.matchemphys.2008.07.030
  10. Malek, Z.; Balek, V.; Garfinkel-Shweky, D.; Yariv, S. J. Them. Anal. 1997, 48, 83. https://doi.org/10.1007/BF01978968
  11. Dean, J. A., Ed.; Lange’s Handbook of Chemistry, 13th ed.; McGraw-Hill: New York, 1985.
  12. Jones, S. A.; Burlitch, J. M.; Duchamp, J. C.; Duncan, T. M. J. Sol-Gel Sci. Technol. 1999, 15, 201. https://doi.org/10.1023/A:1008728724009
  13. Douy, A. J. Sol-Gel Sci. Technol. 2002, 24, 221. https://doi.org/10.1023/A:1015332607551
  14. Almeida, R. M.; Vasconcelos, H. C.; Goncalves, M. C.; Santos, L. F. J. Non-Cryst. Solids 1998, 65, 232.
  15. Earnesy, C. M. Thermochim. Acta 1983, 63, 291. https://doi.org/10.1016/0040-6031(83)80326-8
  16. Boutinaud, P.; Mahiou, R.; Cousseins, J. C. J. Lumin. 1997, 72-74, 318. https://doi.org/10.1016/S0022-2313(96)00172-X

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