Runoff Characteristics of Heavy Metals from a Parking Lot by Rainfall

주차장 지역의 강우에 의한 Pb와 Zn의 유출 특성

  • Im, Jong-Kwon (Department of Environmental Health, School of Public Health, Seoul National University) ;
  • Son, Hyun-Seok (Department of Environmental Health, School of Public Health, Seoul National University) ;
  • Kim, Sung-Keun (Department of Environmental Health, School of Public Health, Seoul National University) ;
  • Zoh, Kyung-Duk (Department of Environmental Health, School of Public Health, Seoul National University)
  • 임종권 (서울대학교 보건대학원 환경보건학과) ;
  • 손현석 (서울대학교 보건대학원 환경보건학과) ;
  • 김성근 (서울대학교 보건대학원 환경보건학과) ;
  • 조경덕 (서울대학교 보건대학원 환경보건학과)
  • Received : 2010.07.05
  • Accepted : 2010.09.13
  • Published : 2010.11.30

Abstract

Runoff from a parking lot can be highly contaminated nonpoint source due to the impermeability of rainwater. This study presented runoff characteristics of heavy metals especially Zn and Pb from a parking lot during total 17 rain events. Monitoring results showed the first flush phenomenon within 30 min was observed in all rain events, but the event mean concentration (EMC) did not clearly show the characteristics of runoff. The ranges of Pb and Zn was $4{\sim}201{\mu}g/L$ and $131{\sim}672{\mu}g/L$, respectively, and the runoff mass of Zn and Pb was highly to related with the flow rate, and runoff coefficient of rain. The runoff mass of Zn was greater than that of Pb in all events. The runoff mass of Pb was highly correlated with the amount of TSS, and TSS and DOC were was related with the mass of Zn. This result implies that Pb and Zn are mainly existed in the particulate form. The results can be used to as meaningful data in the management of nonpoint source, and in the management in the runoff catchment in the parking lot.

Keywords

References

  1. 김이형, 이선하(2005). 주차장 및 교량 강우유출수의 중금속 오염물질 특성과 동적 EMCs. 수질보전 한국물환경학회지, 21(4), pp. 385-392.
  2. 이소영, 이은주, 김철민, 손현근, Marla C. Maniquiz, 손영규, 강회만, 김지형, 김이형(2007). 고속도로 영업소지역의 강우유출수내 중금속 유출 특성. 수질보전 한국물환경학회지, 23(6), pp. 945-950.
  3. 환경부(2008). 환경백서. http://ekp.me.go.kr/ekc/.
  4. APHA, AWWA, WPCF (1998). Standard methods for the examination of water and wastewater. 20th American Public Health Association/American Water Works Association/Water Pollution Control Federation, Washington, DC, USA.
  5. Bach, P. M., MacCarthy, D. T., and Deletic, A. (2010). Redefining the Stormwater first flush phenomenon. Water Res., 44, pp. 2487-2498. https://doi.org/10.1016/j.watres.2010.01.022
  6. Christensen, E. R. and Guinn, V. P. (1979). Zinc from auto-mobile tires in urban runoff, J. Environ. Engineer. Division ASCE, 105, pp. 165-168.
  7. Deletic, A, (1998). The fist flush load of urban surface runoff. Water Res., 32. pp. 2462-2470. https://doi.org/10.1016/S0043-1354(97)00470-3
  8. Dong, A., Chesters, G., and Simsiman, G. V. (1984). Metal composition of soil, sediments and urban dust and dirt samples from the Menomonee river watershed, Wisconsin. USA. Water, Air and Soil Pollution, 22, pp. 257-275.
  9. Gupta, K. and Saul, A. J. (1996). Specific relationships for the first flush load in combined sewer flows. Water Res., 30, pp. 1244-1252. https://doi.org/10.1016/0043-1354(95)00282-0
  10. Harrrison, R. M., Laxen, D. P., and Wilson, S,. J. (1981). Chemical associations of lead, cadium, copper and zinc in street dusts and roadside soil. Environ. Sci. Technoll., 15, pp, 1378-1383. https://doi.org/10.1021/es00093a013
  11. Kayhanian, M., Suverkropp C., Ruby A., and Tsay K. (2007). Characterization and prediction of highway runoff constituent event mean concentration. J. of Environ. Management, 85, pp. 279-295. https://doi.org/10.1016/j.jenvman.2006.09.024
  12. Kim, L. H. (2003). Determination of event mean concentrations and first flush criteria in urban runoff. Kor. Environ. Eng. Research, 8(4), pp. 163-176. https://doi.org/10.4491/eer.2003.8.4.163
  13. Kim, L. H., Kayhanian, M., Zoh, K. D., and Stenstrom, M. K. (2005). Modeling of highway stormwater runoff. Sci. Tot. Environ., 348. pp. 1-18. https://doi.org/10.1016/j.scitotenv.2004.12.063
  14. Kim, L. H., Ko, S. O., Jeong, S., and Yoon, J. (2007). Cha-racteristicsof washed-off pollutants and dynamic EMCs in parking lots and bridges during a Storm. Sci. Tot. Environ., 376, pp. 178-184. https://doi.org/10.1016/j.scitotenv.2006.12.053
  15. Lee, J. H., Bang, K. W., Ketchum, L. H., Choe, J. S., and Yu, M. J. (2002). First flush analysis of urban storm runoff. Sci. Tot. Environ., 293. pp. 163-175. https://doi.org/10.1016/S0048-9697(02)00006-2
  16. Lee. P. K., Baillif, P., and Touray, J. C. (1997). Geochemical behaviour and relative mobility of metal (Mn, Cd, Zn and Pb) in recent sediments of retention pond along the A-71 motorway in slogne, Frence. Environ. Geol., 32(2), pp. 142-152. https://doi.org/10.1007/s002540050203
  17. Liebens, J. (2001). Heavy metal contamination of sediments in stotmwater management systems: the effect of land use, particle size, and age. Environ. Geol., 41, pp. 341-351. https://doi.org/10.1007/s002540100392
  18. Ma, J. S., Khan, S., Li, Y. X., Kim, L. H., Ha, S., Lau, S. L., Kayhanian, M., and Stenstrom, M. K. (2002). First f1ush phenomena for highways: how it can be meaningfully defined. Proceedings of 9th International Conferenceon Urban Drainage, September, Portland, Oregon
  19. McKenzie, E. R., Money, J. E., Green, P. E., and Young, T. M. (2009). Metals associated with stormwater-relevant brake and tird samples. Sci. Tot. Environ., 407, pp. 5855-5860. https://doi.org/10.1016/j.scitotenv.2009.07.018
  20. Rebecca, S. S., John, C. C., and David, R. A. (2002). Treatment of parking lot stormwater using a stormtreat system. Environ. Sci. Technol., 36, pp. 4441 -4446. https://doi.org/10.1021/es020797p
  21. Sansalone. J. J. and Bushbreger. S. G. (1997). Partitioning and first flush of meta1s in urban roadway Storm water. J. Environ. Eng., 123(2), pp. 134-143. https://doi.org/10.1061/(ASCE)0733-9372(1997)123:2(134)
  22. Taebi, A. and Droste, R. L. (2004). First f1ush pollution load of urbanstorm wqter runoff. J. Environ. Engineer., 3, pp. 301-309.
  23. Ujevic. I., Odzak, N., and Baric, A. (2000). Trace metal accumulation in different grain size fractions of the sediments form a semi-enclosed bay heavily contaminated by urban and industrial wastewaters. Water Res., 34, pp. 3055-3061. https://doi.org/10.1016/S0043-1354(99)00376-0