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Vertical Change in Extinction and Atmospheric Particle Size in the Boundary Layers over Beijing: Balloon-borne Measurement

  • Chen, Bin (State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics (LASG), Institute of Atmospheric Physics, Chinese Academy of Sciences) ;
  • Shi, Guang-Yu (State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics (LASG), Institute of Atmospheric Physics, Chinese Academy of Sciences) ;
  • Yamada, Maromu (Center for Innovation, Kanazawa University) ;
  • Zhang, Dai-Zhou (Faculty of Environmental and Symbiotic Sciences, Prefectural University of Kumamoto) ;
  • Hayashi, Masahiko (Department of Earth System Science, Graduate School of Science, Fukuoka University) ;
  • Iwasaka, Yasunobu (Frontier Science Organization, Kanazawa University)
  • Received : 2010.05.26
  • Accepted : 2010.07.23
  • Published : 2010.12.31

Abstract

Aerosol size and number concentration were observed in the atmospheric boundary layer over Beijing (from near the ground to 1,200 m) on March 15 (a clear day) and 16 (a dusty day), 2005. The results were further compared with lidar measurements in order to understand the dependency of extinction on the particle size distribution and their vertical changes. The boundary layer atmosphere was composed of several sub-layers, and a dry air layer appeared between 400 and 1,000 m under the influence of dust event. In this dry air layer, the concentration of the fine-mode particles (diameter smaller than $1.0\;{\mu}m$) was slightly lower than the value on the clear day, while the concentration of coarse-mode particles (diameter larger than $1.0\;{\mu}m$) was remarkably higher than that on the clear day. This situation was attributed to the inflow of an air mass containing large amounts of Asian dust particles and a smaller amount of fine-mode particles. The results strongly suggest that the fine-mode particles affect light extinction even in the dusty atmosphere. However, quantitatively the relation between extinction and particle concentration is not satisfied under the dusty atmospheric conditions since laser beam attenuates in the atmosphere with high concentration of particles. Laser beam attenuation effect becomes larger in the relation between extinction and coarse particle content comparing the relation between extinction and fine particle content. To clarify this problem technically, future in situ measurements such as balloon-borne lidar are suggested. Here extinction was measured at 532 nm wavelength. Measurements of extinction at other wavelengths are desired in the future.

Keywords

References

  1. An, J., Zhang, R., Han, Z. (2000) Seasonal changes oftotal suspended particles in the air of 15 big cities innorthern parts of China. Climatic Environment Research5(1), 25-29. (in Chinese)
  2. Baik, N., Kim, Y.P., Moon, K.C. (1996) Visibility studyin Seoul, 1993. Atmospheric Environment 30, 2319-2328. https://doi.org/10.1016/1352-2310(95)00443-2
  3. Chan, Y.C., Simpson, R.W., Mctainsh, G.H., Vowles, P.D.,Cohen, D.D., Bailey, G.M. (1997) Characterization ofchemical species in $PM_{2.5}\;and\;PM_{10}$ aerosols in Brisbane,Australia. Atmospheric Environment 31, 3773-3785. https://doi.org/10.1016/S1352-2310(97)00213-6
  4. Chan, Y.C., Simpson, R.W., Mctainsh, G.H., Vowles, P.D.,Cohen, D.D., Bailey, G.M. (1999) Source apportionmentof visibility degradation problems in Brisbane(Australia) using the multiple linear regression techniques.Atmospheric Environment 33, 3237-3250. https://doi.org/10.1016/S1352-2310(99)00091-6
  5. Charlson, R.J., Schwartz, S.E., Hales, J.M., Cess, R.D.,Coakley, J.A., Hansen, J.E., Hofmann, D.J. (1992) Climateforcing by anthropogenic aerosols. Science 255,423-430. https://doi.org/10.1126/science.255.5043.423
  6. Dockery, D.W., Pope, C.I. (1994) Acute respiratory effectsof particulate air Pollution. Annual Review of PublicHealth 15, 107-132. https://doi.org/10.1146/annurev.pu.15.050194.000543
  7. Donaldson, K., Li, X.Y., MacNee, W. (1998) Ultra-fine(nanometer) particle mediated lung injury. Journal ofAerosol Science 29, 553-560. https://doi.org/10.1016/S0021-8502(97)00464-3
  8. Hayashi, M., Iwasaka, Y., Watanabe, M., Shibata, T.,Fujiwara, M., Adachi, H., Sakai, T., Nagatani, M.,Gernandt, H., Neuber, R., Tsuchiya, M. (1998) Sizeand number concentration of liquid PSCs: Balloonbornemeasurements at $Ny-{\AA}lesund$, Norway in winterof 1994/95. Journal of the Meteorological Society ofJapan 76, 549-560. https://doi.org/10.2151/jmsj1965.76.4_549
  9. Jacobson, M.Z. (2001) Global direct radiative forcing dueto multicomponent anthropogenic and natural aerosols.Journal of Geophysical Research 106, 1551-1568. https://doi.org/10.1029/2000JD900514
  10. Koschmieder, H. (1924) Theorie der horizontalen Sichtwcete,Bcetr. Physical Atmosphere 12, 33-53.
  11. Larson, S.M., Cass, G.R. (1989) Characteristics of summermiddy low visibility events in the Los Angeles area.Environmental Science & Technology 23, 281. https://doi.org/10.1021/es00180a003
  12. Li, B.G., Ran, Y., Tao, S. (2008) Seasonal variation andspatial distribution of atmospheric aerosols in Beijing.Acta Scientiae Circumstantiae 28(7), 1425-1429. (inChinese)
  13. Liu, X., Shao, M. (2004) The analysis of sources of ambientlight extinction coefficient in summer time of Beijingcity. Acta Scientiae Circumstantiae 24(2), 185-189. (in Chinese)
  14. Liu, Y., Zhou, M. (1999) The internal variation of mineralaerosols in the surface air over Beijing and the EastChina Sea. Acta Scientiae Circumstantiae 19(06), 642-647. (in Chinese)
  15. Matsuki, A., Iwasaka, Y., Shi, G.-Y., Chen, H.-B., Osada,K., Zhang, D., Kido, M., Inomata, Y., Kim, Y.-S.,Trochkine, D., Nishita, C., Yamada, M., Nagatani, T.,Nagatani, M., Nakata, H. (2005) Heterogeneous sulfateformation on dust surface and its dependence on mineralogy:balloon-borne observations from balloon-bornemeasurements in the surface atmosphere of Beijing,China. Water, Air, & Soil Pollution: Focus 5(3-6), 101-132. https://doi.org/10.1007/s11267-005-0730-3
  16. Peundorf, R. (1957) Tables of the refractive index forstandard and the Rayleigh scattering coefficient for thespectral region between 0.2 and 20.0 ${\mu}s$ and their applicationto atmospheric optics. Journal of the OpticalSociety of America 47, 176-182. https://doi.org/10.1364/JOSA.47.000176
  17. Prospero, J.M. (1999) Long range transport of mineraldust in the global atmosphere: Impact of African duston the environment of the southeastern United States.Proceedings of the National Academy of Sciences USA96, 3396-3403. https://doi.org/10.1073/pnas.96.7.3396
  18. Seinfeld, J.H., Pandis, S.N. (1998) Atmospheric Chemistryand Physics: From Air Pollution to Climate Change(John Wiley, New York), pp. 724-743.
  19. Shimizu, A., Sugimoto, N., Matsui, I., Arao, K., Uno, I.,Murayama, T., Kagawa, N., Aoki, K., Uchiyama, A.,Yamazaki, A. (2004) Continuous observations of Asiandust and other aerosols by polarization lidars in Chinaand Japan during ACE-Asia. Journal of GeophysicalResearch 109, D19S17, doi:10.1029/2002JD003253.
  20. Song, Y., Tang, X.Y., Fang, C., Zhang, Y.H., Hu, M.,Zeng, L.M., Li, C.C., Mao. J.T. (2003) Relationshipbetween the visibility degradation and particle pollutionin Beijing. Acta Scientiae Circumstantiae 23(4), 468-471. (in Chinese)
  21. Sugimoto, N., Uno, I., Nishikawa, M., Shimizu, A., Matsui,I., Dong, X.H., Chen, Y., Quan, H. (2003) Recordheavy Asian dust in Beijing in 2002: Observations andmodel analysis of recent events. Geophysical ResearchLetters 30(12), 1640, doi:10.1029/2002GL016349.
  22. Wang, J.L., Liu, X.L. (2006) The discuss on relationshipbetween visibility and mass concentration of $PM_{2.5}$ inBeijing. Acta Meteorologica Sinica 64(2), 221-228.(in Chinese)
  23. Wang, W., Tang, D., Liu, H., Yue, X., Pan, Z., Ding, Y.(2000) Research on current pollution status and pollutioncharacteristics of $PM_{2.5}$ in China. Research ofEnvironmental Sciences 13(1), 1-5.
  24. Wu, M., Niu, Z., Qiao, Y., Wu, C. (2009) Aerosol typesand its affecting factors over Beijing: Based on MODISdata. GEO-INFORMATION SCIENCE 11(4), 541-548. (in Chinese) https://doi.org/10.3724/SP.J.1047.2009.00541
  25. Xu, J., Zhang, X., Yan, P., Ding, G., Xu, X. (2008) Observationalstudy of aerosol extinction property duringdust weather in background area. Meteorological Scienceand Technology 36(6), 679-685. (in Chinese)
  26. Yamashita, K., Hayashi, M., Irie, M., Yamamoto, K.,Saga, K., Ashida, M., Shiraishi, K., Okabe, K. (2005)Amount and state of mineral particles in the uppermixed layer and the lower free troposphere over Mt.Raizan, southwestern Japan: unmanned airplane measurementsin the Spring of 2003. Journal of the MeteorologicalSociety of Japan 83A, 121-136. https://doi.org/10.2151/jmsj.83A.121
  27. Yan, F.Q., Hu, H.L., Zhou, J. (2003) Measurement ofnumber density distribution and imaginary part of refractiveindex of aerosol particles. Acta Optica Sinia23(7), 855-859. (in Chinese)
  28. Yuan, Y., Liu, D., Che, R., Dong, X. (2007) Research onthe pollution situation of atmospheric particulates duringAutumn in Beijing city. Ecology and Environment16(1), 18-25. (in Chinese)
  29. Zhang, R., Xu, Y., Han, Z. (2003) Inorganic chemicalcomposition and source signature of $PM_{2.5}$ in Beijingduring ACE2 Asia period. Chinese Science Bulletin48(7), 730-733. (in Chinese)
  30. Zhang, R., Han, Z., Shen, Z., Cao, J. (2008) Concentrationsand elemental composition of aerosol particlesfor a dust storm event in Beijing, Advances in AtmosphericSciences (25), 89-95.

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