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Removal of Gaseous Toluene using a Plate-type Dielectric Barrier Discharge Reactor

평판형 전극으로 구성된 유전체 배리어 방전 반응기를 이용한 톨루엔 저감 특성

  • Park, Jae-Hong (Department of Mechanical Engineering, Yonsei University) ;
  • Jo, Yoon-Shin (Department of Mechanical Engineering, Yonsei University) ;
  • Yoon, Ki-Young (Department of Mechanical Engineering, Yonsei University) ;
  • Byeon, Jeong-Hoon (Digital Printing Division, Samsung Electronics Co., Ltd.) ;
  • Hwang, Jung-Ho (Department of Mechanical Engineering, Yonsei University)
  • 박재홍 (연세대학교 기계공학과) ;
  • 조윤신 (연세대학교 기계공학과) ;
  • 윤기영 (연세대학교 기계공학과) ;
  • 변정훈 (삼성전자주식회사 디지털프린팅사업부) ;
  • 황정호 (연세대학교 기계공학과)
  • Published : 2008.12.31

Abstract

A plate-type dielectric barrier discharge (DBD) reactor was designed and tested for removal of gaseous toluene. The DBD reactor consisted of 9 parallel plate electrodes, four of which were grounded. An AC voltage of rectangular waveform ($5{\sim}8.5kV$, $60{\sim}1,000Hz$), was applied to the other five electrodes. The gaseous toluene passed through the DBD reactor and its concentration was measured by a real-time gas analyzer. The carbon monoxide (CO) and carbon dioxide ($CO_2$) which were produced by decomposition of toluene in the DBD reactor, were sampled and analyzed by a micro gas chromatography. The maximum toluene removal efficiency was 51.4%.

Keywords

References

  1. 김관태, 김용호, 차민석, 송영훈, 김석준, 류정인 (2004) DBD 반응기에서 플라즈마 방전형태에 따른 PFCs 가스의 분해 특성, 한국대기환경학회지, 20(5), 625-632
  2. 김상환, 강태성, 양희성, 브트린뉴이, 박형상 (2006) 알루미나 에 담지한 백금 촉매상에서 휘발성 유기화합물 톨루엔 및 톨루엔+자일렌의 저온산화, 한국대기환경학회지, 22(6), 799-807
  3. 김상국, 장예림 (2008) 활성탄소섬유 흡착bed에서의 톨루엔 흡착특성, 한국대기환경학회지, 24(2), 220-228 https://doi.org/10.5572/KOSAE.2008.24.2.220
  4. 박재윤, 정장근, 김종석, 하현진(2005) 고주파 플라즈마 시스 템에 의한 디젤기관의 배기가스 특성, 한국조명. 전기설비학회논문지, 19(5), 109-113 https://doi.org/10.5207/JIEIE.2005.19.5.109
  5. 이주상, 김신도, 김광영, 김종호 (1995) 연면방전의 플라즈마 화학처리에 의한 유해가스제어 성능에 관한 연구, 한국대기보전학회지, 11(2), 185-190
  6. 전상구, 신대현, 문승현 (2004) 저온 플라즈마/촉매 복합 시 스템을 이용한 유해가스물질들의 저감, 한국자동 차공학회 춘계학술대회 논문집, I, 221-226
  7. 정재우, 이용환, 박경렬 (2002) 무성방전내에서 톨루엔 제거 에 미치는 운전변수의 영향, 한국대기환경학회지, 18(3), 173-182
  8. 최영석, 서동범, 이원남, 송영훈(1999) 저온 플라즈마 반응기의 톨루엔 , 프로판 및 에틸렌 제거 특성 및 반응 메커니즘, 대한기계학회 추계학술대회논문집, B, 145-150
  9. Abdel-Salam, M., A. Hashem, A. Yehia, A. Mizuno, A. Turky, and A. Gabr (2003) Characteristics of corona and silent discharges as influenced by geometry of the discharge reactor, J. Phys. D: Appl. Phys., 36, 252-260 https://doi.org/10.1088/0022-3727/36/3/306
  10. Delagrange, S., Pinard, L., and Tatibouet, J.M. (2006) Combination of a non-thermal plasma and a catalyst for toluene removal from air: Manganese based oxide catalysts, Applied Catalysis B: Environmental 68, 92-98 https://doi.org/10.1016/j.apcatb.2006.07.002
  11. Falkenstein, Z. (1998) Application of dielectric barrier discharge, 12th Int. Conf on High-Energy Particle Beams, Beams'98, Haifa, Israel, June pp. 7-12, 117 -120
  12. Guo, Y.F., D.Q. Ye, K.F. Chen, J.C. He, and W.L. Chen (2006) Toluene decomposition using a wire-plate dielectric barrier discharge reactor with manganese oxide catalyst in situ, Journal of Molecular Catalysis A: Chemical, 245, 93-100 https://doi.org/10.1016/j.molcata.2005.09.013
  13. Higashi, M., S. Uchida, N. Suzuki, and K. Fujii (1992) Soot elimination and $NO_{x}$ and $SO_{x}$ reduction in dieselengine exhaust by a combination of discharge plasma and oil dynamics, IEEE Trans. Plasma Sci., 20 (1), 1-12 https://doi.org/10.1109/27.120185
  14. Hinds W.C. 1999. Aerosol technology. New York: John- Wiley&Sons
  15. Lu, B., X. Zhang, X. Yu, T. Feng, and S. Yao (2006) Catalytic oxidation of benzene using DBD corona discharges, J. Hazard. Mater., 137, 633-637 https://doi.org/10.1016/j.jhazmat.2006.02.012
  16. Magureanu, M., N.B. Mandache, P. Eloy, E.M. Gaigneaux, and V.I. Parvulescu (2005) Plasma-assisted catalysis for volatile organic compounds abatement, Applied Catalysis B: Environmental, 61, 12-20 https://doi.org/10.1016/j.apcatb.2005.04.007
  17. Mizuno, A. (2000) Electrostatic precipitation, IEEE Trans. Dielectrics Electrical Insulation, 7, 615-624 https://doi.org/10.1109/94.879357
  18. Rosocha, L.A., J.J. Coogan, and M. Kang (1994) Use of silent electrical discharges for environmental remediation, IEEE Int. Conf., 88, IE4
  19. Yamamoto, K., M. Yukimura, S. Kambara, H. Moritomi, T. Yamashita, and T. Maruyama (2004) Effect of O2 on NO removal by ammonia radical injection using one-cycle sinusoidal power source, Thin Solid Films, 457, 39-43 https://doi.org/10.1016/j.tsf.2003.12.011
  20. Yamamoto, T., M. Okubo, T. Nagaoka, and K. Hayakawa (2000) Simultaneous removal of NOx and SOx in flue gas emission using plasma-chemical hybrid process, Ind. Appl. Conf., Conf. Rec. 2000, IEEE, 1, 641-647