Journal of Korean Society for Atmospheric Environment (한국대기환경학회지)

Korean Society for Atmospheric Environment (한국대기환경학회)
권호 표지
DOI QR코드

DOI QR Code

Seasonal and Diurnal Variations of Surface Ozone at Ieodo in the East China Sea

이어도 해양과학기지의 오존농도의 계절변화와 일변화 특징

  • Shin, Beom-Cheol (Department of Earth & Environmental Sciences, Korea University) ;
  • Lee, Mee-Hye (Department of Earth & Environmental Sciences, Korea University) ;
  • Lee, Jae-Hak (Division of Climate and Environment Research, Korean Ocean Research and Development Institute) ;
  • Shim, Jae-Seol (Division of Coastal and Harbor Engineering Research, Korean Ocean Research and Development Institute)
  • 신범철 (고려대학교 지구환경과학과) ;
  • 이미혜 (고려대학교 지구환경과학과) ;
  • 이재학 (한국해양연구원 해양환경연구본부) ;
  • 심재설 (한국해양연구원 연안개발연구본부)
  • Published : 2007.12.31
Download PDF
⟨ Previous Next ⟩

Abstract

We examined diurnal and seasonal variations of ozone ($O_3$) concentrations and its relation to meteorological parameters observed at the Ieodo Ocean Research Station ($32.07^{\circ}N$, $125.10^{\circ}E$, 36 m above sea level) during June 2003 and May 2005. Over the 2-year period, the mean ozone concentration was $49.5{\pm}15.5\;ppbv$. Ozone concentrations show great variability with a monthly mean up to 68.2 ppbv in May 2005 and seasonal variations with being highest in spring and fall, and lowest in summer. However, the amplitude of diurnal variation was less than ${\sim}4\;ppbv$ with a maximum at $3{\sim}4\;p.m.$ and minimum at $7{\sim}8\;a.m.$ HYSPLIT backward air trajectory indicated that the air masses with higher ozone came from the north or northwest and those with lower ozone arrived mainly via southerly or southeasterly. Ozone distributions at Ieodo Ocean Research Station were observed to be significantly impacted by long-range transport and regional scale air circulation.

Keywords

References

  1. 김영성 (1996) 1991-1993년 사이 우리나라의 오존 농도 변화, 한국대기보전학회지, 12(1), 55-66
  2. 김용표, 김진영, 박세옥, 김성주, 심상규, 문길주, 박경윤, 허철구(1996) 고산에서의 1994년 3-4월 측정연구 : (II) 기체상 대기오염물질의 특성, 한국대기보전학회지, 12(1), 91-99
  3. 박경윤, 이호근, 서명석, 장광미, 강창희, 허철구, 김영준(1994) 제주도 고산 측정소에서의 대기오염 배경농도 측정 및 분석, 한국대기보전학회지, 10(4), 252-259
  4. Ayers, G.P., H. Granek, and R. Boers (1997) Ozone in the marine boundary layer at Cape Grim Model simulation, J. Atmos. Chem., 27, 179-195 https://doi.org/10.1023/A:1005828930552
  5. Bremaud, P.J., F. Taupin, A.M. Thomson, and N. Chaumerliac (1998) Ozone nighttime recovery in the marine boundary layer: measurements and simulation of the ozone cycle at Reunion Island, J. Geophys. Res., 103, 3463-3473 https://doi.org/10.1029/97JD01972
  6. Cvitas, T., M. Furger, R. Girgzdiene, L. Haszpra, N. Kezele, L. Klasinc, A. Planinsek, M. Pompe, A.S.H. Prevot, H.E. Scheel, and E. Schuepbach (2004) Spectral analysis of boundary layer ozone data from the EUROTRAC TOR network, J. Geophys. Res., 109, D02302, doi:10.1029/2003JD003727
  7. Derwent, R.G., P.G. Simmonds, S. Seuring, and C. Cimmer (1998) Observation and interpretation of the seasonal cycles in the surface concentrations of ozone and carbon monoxide at Mace Head, Ireland from 1990 to 1994, Atmos. Environ., 32, 144-157
  8. Draxler, R.R. and G.D. Rolph (2003) HYSPLIT (Hybrid Single -Particle Lagrangian Integrated Trajectory) Model access via NOAA ARL READY. Website http:// www.arl.noaa.gov/ready/hysplit4.html. NOAA Air Resources Laboratory, Silver Spring, MD
  9. Fishman, J. and V.G. Brackett (1997) The climatological distribution of tropospheric ozone derived from satellite measurements using version 7 Total Ozone Mapping Spectrometer and Stratospheric Aerosol and Gas Experiment data sets, J. Geophys. Res., 102, 19275-19278 https://doi.org/10.1029/97JD01373
  10. Ghim, Y.S. and Y.-S. Chang (2000) Characteristics of ground- level ozone distributions in Korea for the period of 1990-1995, J. Geophys. Res., 105, 8877- 8890 https://doi.org/10.1029/1999JD901179
  11. Jaffe, D.A., R.E. Honrath, L. Zhang, H. Akimoto, A. Shimizu, H. Mukai, K. Murano, S. Hatakeyama, and J. Merrill (1996) Measurements of NO, NOy, CO and $O_3 $and estimation of the ozone production rate at Oki Island, Japan, during PEM-West, J. Geophys. Res., 101, 2037-2048 https://doi.org/10.1029/95JD01699
  12. Kajii, Y., K. Someno, H. Tanimoto, J. Hirokawa, H. Akimoto, T. Katsuno, and J. Kawara (1998) Evidence of the seasonal variation of photochemical activity of tropospheric ozone: continuous observation of ozone and CO at Happo, Japan, Geophys. Res. Lett., 25, 3305-3508 https://doi.org/10.1029/98GL02563
  13. Lelieveld, J. and F.J. Dentener (2000) What controls tropospheric ozone?, J. Geophys. Res., 105, 3531-3551 https://doi.org/10.1029/1999JD901011
  14. Monks, P.S., G. Holland, G. Salisbury, S.A. Penkett, and G. P. Ayers (2000) A seasonal comparison of ozone photochemistry in the remote marine boundary layer, Atmos. Environ., 34, 2547-2561 https://doi.org/10.1016/S1352-2310(99)00504-X
  15. Oltmans, S.J. and W.D. Komhyr (1986) Surface ozone distributions and variations from 1973-1984 measurements at the NOAA geophysical monitoring for climatic change baseline observatories, J. Geophys. Res., 91, 5229-5236 https://doi.org/10.1029/JD091iD04p05229
  16. Oltmans, S.J. and H. Levy III (1994) Surface ozone measurements from a global network, Atmos. Environ., 28, 9-24 https://doi.org/10.1016/1352-2310(94)90019-1
  17. Parrish, D.D., M. Trainer, J.S. Holloway, J.E. Yee, M.S. Warshawsky, and F.C. Fehsenfeld (1998) Relationships between ozone and carbon monoxide at surface sites in the North Atlantic Ocean, J. Geophys. Res., 103(D11), 13357-13376 https://doi.org/10.1029/98JD00376
  18. Penkett, S.A., N.J. Blake, P. Lightman, A.R.W. Marsh, P. Anwyl, and G. Butcher (1993) The seasonal variation of non-methane hydrocarbons in the free troposphere over the North Atlantic Ocean: possible evidence for extensive reaction of hydrocarbons with the nitrate radical, J. Geophys. Res., 98, 2865- 2885 https://doi.org/10.1029/92JD02162
  19. Pochanart, P., J. Hirokawa, Y. Kajii, H. Akimoto, and M. Nakao (1999) The influence of regional-scale anthropogenic activity in the northeast Asia on seasonal variations of surface ozone and its precursors observed at Oki, Japan, J. Geophys. Res., 104, 3621-3632 https://doi.org/10.1029/1998JD100071
  20. Ridley, B., J. Walega, G. Hübler, D. Montzka, E. Atlas, D. Hauglustaine, F. Grahek, J. Lind, T. Campos, R. Norton, J. Greenberg, S. Schauffler, S. Oltmans, and S. Whittlestone (1998) Measurements of NOx and PAN and estimates of $O_3 $production over the seasons during Mauna Loa Observatory Photochemistry Experiment 2, J. Geophys. Res., 103, 8323-8339 https://doi.org/10.1029/98JD00075
  21. Roelofs, G.-J., J. Lelieveld, and R. van Dorland (1997) A three-dimensional chemistry/general circulation model simulation of anthropogenically derived ozone in the troposphere and its radiative climate forcing, J. Geophys. Res., 102, 23389-23401 https://doi.org/10.1029/97JD02210
  22. Seinfeld, J.H. and S.N. Pandis (1998) Atmospheric Chemistry and Physics: From Air Pollution to Climate Change, J. Wiley & Sons, New York, 1326 pp.
  23. Sunwoo, Y., G.R. Chamichael, and H. Ueda (1994) Characteristics of background surface ozone in Japan, Atmos. Environ., 28, 25-37 https://doi.org/10.1016/1352-2310(94)90020-5
  24. Watanabe, K., Y. Nojiri, and S. Kariya (2005) Measurements of ozone concentrations on a commercial vessel in the marine boundary layer over the northern North Pacific Ocean, J. Geophys. Res., 110, D11310, doi :10.1029/2004JD005514
  25. Winkler, P. (1988) Surface ozone over the Atlantic, J. Atmos. Chem., 7, 73-91 https://doi.org/10.1007/BF00048255

Cited by

  1. Photochemical Air Pollution of Seoul in the Last Three Decades vol.29, pp.4, 2013, https://doi.org/10.5572/KOSAE.2013.29.4.390
  2. at Ieodo Ocean Research Station vol.29, pp.6, 2013, https://doi.org/10.5572/KOSAE.2013.29.6.701