Environmental Engineering Research

Korean Society of Environmental Engineers (대한환경공학회)
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RESEARCH PAPERS : SOLUBILITIES OF AM, U, NP AND PU IN GRANITIC GROUNDWATER

  • Keum, Dong-Kwon (Korea Aromic Energy Research Institute (KAERI)) ;
  • Lee, Han-Soo (Korea Aromic Energy Research Institute (KAERI)) ;
  • Lee, Chang-Woo (Korea Aromic Energy Research Institute (KAERI)) ;
  • Volker Metz (Institute for Nuclear Waste Management, Research Center Karlsruhe)
  • Published : 2004.04.30
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References

  1. Martinez-Esparza, A, Esteben, J.A, Quinones, J., de Pablo, J., Casas, I., Gimenez, J., Clarens, F., Rovira, M., Merino, J., Cera, E., Bruno, J. and Ripoll, S., Modeling spent fuel and HLW behavior in repository conditions, ENRESA, Publication technical 08/2002 (2002)
  2. Dormuth, K.W., Assessment of the Canadian Nuclear Fuel Disposal Concept, Proceeding of Symposium on Safety Assessment of Radioactive Waste Repositories, OECDINEA, pp.211-218 (1993)
  3. Golder Associates, Performance Evaluations Related to Area Characterization of Crystalline Rock, Golder Associates, Office Crystalline Repository Division, OH, BMI/OCRD-27 (1988)
  4. Nagra, Project Gewahr 1985, Nagra, Baden, Project Report, NGB 85-09 (1985)
  5. PNC, Research and Development on Geological Disposal of High-Level Radioactive Waste: Final Progress Report, PNC, Tokyo, Tech. Report, TN1410 93-018 (1992)
  6. SKB, SKB-91; Final Disposal of Spent Nuclear Fuel- Importance of the Bedrock for Safety, SKB, Stockholm, Tech. Report, TR 92-20 (1992)
  7. SKI, SKI Project 90 Summary, SKI, Stockholm, Tech., Report 91-23 (1991)
  8. TVO, Final Disposal of Spent Nuclear Fuel in Finnish Bedrock, YJT, Helsinki, Tech. Report, YJT-92-31E (1992)
  9. Metz, V., Kienzler, B. and Schuessler, W., Geochemical evaluation of different ground-water-host rock systems for radioactive waste disposal, J. Contamin. Hydrology, 61, 265-279 (2003)
  10. Bond, K.A., Heath, T.G., and Tweed, C.J., HATCHES: A Reference Thermodynamic Database for Chemical Equilibrium Studies. Nirex Report NSS/R379, December (1997)
  11. Felmy, A.R., Girvin, D., and Jenne, E.A., MINTEQ: A Computer Program for Calculating Aqueous Geochemical Equilibria, EPA-600/3-84-032, U.S. Environmental Protection Agency, by Battelle, Pacific Northwest Laboratories, Richland, Washington (1984)
  12. Wolery, T.J., Calculation of Chemical Equilibrium between Aqueous Solutions and Minerals: The EQ3/6 Software Package, LLNL, Livermore, CA, UCRL-52658 (1992)
  13. Grenthe, I., Fuger, J., Konings, R.J.M., Lemire, R.J., Muller, A.B., Gregu, C.N. and Wanner, H., Chemical Thermodynamics Series I: Chemical Thermodynamics of uranium: NEA-TDB, OECD, North Holland Elsevier Science Publishers (1992)
  14. Silva, R.J., Bidoglio, G., Rand, M.H., Robouch, P.B., Wanner, H., and Puigdomenech, I., Chemical Thermodynamics Series 2: Chemical Thermodynamics of Americium: NEA-TDB, OECD, North-Holland Elsevier Science Publishers (1995)
  15. Lemire, R.J., Fuger, J., Nitsche, H., Potter, P., Rand, M.H., Rydberg, J., Spahiu, K., Sullivan, J.C., Ullman, W.J., Vitorge, P., and Wanner, H., Chemical Thermodynamics Series 4: Chemical Thermodynamics of Neptunium and Plutonium: NEA-TDB, OECD, North-Holland Elsevier Science Publishers (2001)
  16. Hummel, W., Berner, U., Curti, E., Pearson, F.J., and Thoenen, T., NAGRA/PSI Chemical Thermodynamic Data Base 01/01, Universal Publishers, Parkland (2002)
  17. Grambow, B., Loida, A., Martinez-Esparza, A., Diaz-Arocas, P., de Pablo, J., Paul, J.L., Marx, G., Glatz, J.P., Lemmens, K., Ollila, K. and Christensen, H., Long-term Safety of Radioactive Waste Disposal: Source Term for Performance Assessment of Spent Fuel as a Waste Form, Final Report, Forschungszentrum Karlsruhe, FZKA 6420 (2000)
  18. Keum, D.K. and Hahn, P.S., Application and Development of a Multi-geochemical Reaction Equilibrium Model (MUGREM), Environment Eng. Res. 4, 113-126 (1999)
  19. Keum, D.K., Baik M.H., and Hahn, P.S., Thermodynamic data of Am, Th, U, Np and Pu and their application for HLW disposal, KAERI- KAERI-FZK/INE joint study, Technical report, KAERI/TR-2046/02 (2002)
  20. Bethke, C.M., The Geochemists Workbench. A users guide to Rxn, Acts, Tact, React, and Gtplot. Software package release 3.1, University of Illinois, Urbana-Champaign, USA (2000)
  21. Neck, V., Fanghanel, Th. and Kim, J.I., Aquatische Chemie und Thermodynamische Modellierung von Trivalenten Actiniden, report FZKA 6110, Forschungszentrum Karlsruhe (1998)
  22. Neck, V. and Kim, J.I., Thermodynamics of Tetravalent Actinides: A Critical Assessment of Uncertainties, Actinides2001 Conferences, Hajiyama, Japan (2001)
  23. Takeda, S., Shima, S. and Kimura, H., The aqueous solubility and speciation analysis for uranium, neptunium and selenium by the EQ3/6, JAERI research 95-069 (1995)
  24. Neck, V. and Kim, J.I., Solubility and Hydrolysis of Tetravalent Actinides, Radiochimica. Acta, 89, 1-16 (2001)
  25. Moon, H.C., Equilibrium Ultrafiltration of Hydrolized Thorium(IV) Solutions, Bull. Koran Chem. Soc., 10, p.270 (1989)
  26. Parks, G.A. and Pohl, D.C., Hydrothermal Solubility of Uraninite, Geochim. Cosmochim. Acta, 52, p863 (1988)
  27. Neck, V. and Kim, J.I., An Electrostatic Approach for the Prediction of Actinide Complexation Constants with Inorganic Ligands-Application to Carbonate Complexes, Radiochimica. Acta, 88, 815-822 (2000)
  28. Diaz-Arocas, P. and Grambow, B., Solid-Liquid Phase Equilibria of U(VI) in NaCI Brines, Geochim. Cosmochim Acta, 62, 236-245 (1998)
  29. Finch, J.R., Thermodynamic stabilities of U(Vl) minerals: Estimated and observed relationships, Material research Society. Symposium, 465, 1185-1192 (1997)
  30. Konnecke, Th., Fanghanel, Th., and Kim, J.I., Thermodynamics of Trivalent Actinides in Concentrated Electrolyte Solutions: Modeling the Chloride Complexation of Cm(III), Radiochimica Acta, Vol. 76, 131-135 (1997)
  31. Moll, H., Geipel, G., Metz, W., Bernhard, G., and Nitsche, H., Solubility and Speciation of $(UO_2)_2SiO_42H_2O$ in Aqueous Systems, Radiochimica Acta, 74, 3-7 (1996)
  32. Neck, V., Runde, W., Kim, J.I., and KaneIlakopulos, B., Solid-Liquid Equilibrium Reactions of Neptunium(V) in Carbonate Solution at Different Ionic Strength, Radiochimica Acta, 65, 29-37 (1994)
  33. Neck, V., Fanghanel, Th., and Kim, J.I., Thermodynamics of Neptunium(V) in Concentrated Salt Solutions: Il.Ion Interaction (Pitzer) Parameters for Np(V) Hydrolysis Species and Carbonate Complexes, Radio-chimica. Acta, 69, p.169 (1995)
  34. Neck, V. and Metz, V. (INE/FZK, Germany), (personal communication), (2001)
  35. Neck, V. (INE/FZK, Germany), (personal communication), (2001)

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