Journal of Environmental Science International (한국환경과학회지)

The Korean Environmental Sciences Society (한국환경과학회)
권호 표지
DOI QR코드

DOI QR Code

Polycyclic Aromatic Hydrocarbons in the sediments of Kwangyang Bay on Korea

광양만 유역 퇴적토 중의 다환방향족탄화수소류

  • Published : 2004.06.01
Download PDF
⟨ Previous Next ⟩

Abstract

Polycyclic aromatic hydrocarbons(PAHs) in sediments of Kwangyang bay on Korea, have been investigated by gas chromatography-mass spectrometery (GC/MS). The average content of total PAHs in all samples was 2,211ppb, and the range was from 36 to 22,699ppb. The higher concentrations were found in sediment sampled near Kwangyang iron processing plant, Taeindo. The resulting distributions of PAHs according to the number of aromatic ring and molecular ratios of specific aromatic compounds (phenanthrene, anthracene, fluoranthene and pyrene) have been discussed in terms of sample location, origin of the organic matter. Four, five and six rings of PAHs were mainly found near to Kwangyang iron processing plant, and three and four rings near to Yeosu chemical kombinat This result typically indicated the local characteristics, depending on the origin of PAHs.

Keywords

References

  1. 이종섭, 이문옥, 박일흠, 이삼노, 1997. 광양만권 개발에 따른 해양환경의 변화, 대한토목학회 학술발표회 논문집, 473-476pp.
  2. 김성우, 김윤신, 전준민, 2001, 여천공단내 실내.외 미세분진중의 화학원소 농도 및 발생원 추정에 관한 연구, 대한환경공학회지, 23(2), 305-317.
  3. Magi, E., R. Bianco, C. Ianni and M. Di. Carro, 2002, Distribution of polycyclic aromatic hydrocarbons in the sediments of the Adriatic Sea, Environmental Pollution, 119(1), 91-98. https://doi.org/10.1016/S0269-7491(01)00321-9
  4. 한국해양연구소, 2000, 해양환경 관측 및 개선을 위한 기반기술연구, BSPE 00787-00-1297-1.
  5. Nam, J. J., B. H. Song, K. C. Eam, S. H. Lee and A. Smith, 2003, Distribution of polycyclic aromatic hydrocarbons in agricultural soils in South Korea, Chemosphere, 50, 1281-1289. https://doi.org/10.1016/S0045-6535(02)00764-6
  6. Macias-Zamora, J. V., E. Mendoza-Vega and J. A Villaescusa-Celaya, 2002, PAHs composition of surface marine sediments: a comparison to potential local sources in Todos Santos Bay, B.C., Mexico, Chemosphere, 46(3), 459-468. https://doi.org/10.1016/S0045-6535(01)00069-8
  7. Wu, Y., J. Zhang and Z. Zhu, 2003, Polycyclic aromatic hydrocarbons in the sediments of the Yalujiang Estuary, North China, Marine Pollution Bulletin, 46(5), 619-625. https://doi.org/10.1016/S0025-326X(03)00035-3
  8. 박갑성, 강구영, 염혜정, 1996, PAHs 오염 유해 토양 부지의 생물학적 교정 : 동시 산화, 한국수질보전학회지, 12(3), 245-248.
  9. 박갑성, 1987, 토양에서의 Polycyclic Aromatic Hydrocarbons(PAHs)의 분해, 대한환경공학회지, 9(2), 47-54.
  10. Budzinski, H., I. Jones, J. Bellocq, C. Pierard and P. Garriguses, 1997, Evaluation of sediment contamination by polycyclic aromatic hydrocarbons in the Gironde estuary, Mar. Chem., 58, 85-97. https://doi.org/10.1016/S0304-4203(97)00028-5
  11. Gschwend, P. M. and R. A. Hites, 1981, Fluxes of the polycyclic aromatic compounds to marine and lacustrine sediments in the northeastern United States, Geochim. Cosmochim. Acta., 45, 2359-2367. https://doi.org/10.1016/0016-7037(81)90089-2
  12. Sicre, M. A., J. C. Marty, A. Saliot, X. Aparicio, J. Grimalt and J. Albaiges, 1987, Aliphatic and aromatic hydrocarbons in different sized aerosols over the Mediterranean Sea: Occurrence and origin, Atmos. Environ., 21, 2247-2259. https://doi.org/10.1016/0004-6981(87)90356-8
  13. Colombo, J. C., E. Pelletier, C. Brochu, M. Khalil and J. A Catoggio, 1989, Determination of hydrocarbon sources using n-alkenes and polyaromatic hydrocarbon distribution indexes. Case study: Rio de la Plate, Argentina, Environ. Sci. Technol., 23, 888-894. https://doi.org/10.1021/es00065a019
  14. Benner, B. A., N. P. Bryner, S. A. Wise, G. H. Mulholland, R. C. Lao, and M. F. Fingas, 1990, Polycyclic aromatic hydrocarbons emissions from combustion of crude oil on water, Environ. Sci. Technol., 24, 1418-1427. https://doi.org/10.1021/es00079a018
  15. Benner, B. A., G. E. Gordon and S. A. Wise, 1989, Mobile sources of atmospheric polycyclic aromatic hydrocarbons: A roadway tunnel study, Environ. Sci. Technol., 23, 1269-1278. https://doi.org/10.1021/es00068a014
  16. Wise, S. A., B. A Benner, N. P. Bryner, S. N. Chesler, R. E. Rebbert and M. M. Schantz, 1988, Determination of polycyclic aromatic hydrocarbons in a coal tar standard reference material, Anal. Chem., 60, 887-894. https://doi.org/10.1021/ac00160a012
  17. Williams, P. T., K. D. Bartle and G. E. Andrews, 1986, The relation between polycyclic aromatic compounds in diesel fuels and exhaust particulates, Fuel, 65, 1150-1158. https://doi.org/10.1016/0016-2361(86)90184-5
  18. Masclet, P., M. A. Bresson and G. Mouvier, 1987, Polycyclic aromatic hydrocarbons emmitted by power stations and influence of combustion conditions, Fuel, 66, 556-562. https://doi.org/10.1016/0016-2361(87)90163-3
  19. Nelson, P. F., I. W. Smith, R. J. Tyler and J. C. Mackie, 1988, Pyrolysis of coal at high temperatures, Energy Fuels, 2, 391-400. https://doi.org/10.1021/ef00010a004
  20. Muel, B. and S. Saguem, 1985, Determination of 23 polycyclic aromatic hydrocarbons in atmospheric particulate matter of Paris area and photolysis by sun light, Environ. Sci. Technol., 19, 111-131.
  21. Yang, S. Y. N., D. W. Connell, D. W. Hawker and S. I. Kayal, 1991, Polycyclic aromatic hydrocarbons in air, soil, and vegetation in the viciniyt of an urban roadway, Sci. Total Environ 102, 229-240. https://doi.org/10.1016/0048-9697(91)90317-8