DOI QR코드

DOI QR Code

Synthesis of W18O49 Phase by Carbothermal Reduction of Tungsten Oxide and its Field Emission Characteristics

  • Yang, Hyo-Seung (Nano-Materials Research Center, Korea Institute of Science and Technology, Division of Materials Science and Engineering, Korea University) ;
  • Park, Hoon (Nano-Materials Research Center, Korea Institute of Science and Technolog) ;
  • Kim, Hyoung-chul (Nano-Materials Research Center, Korea Institute of Science and Technolog) ;
  • Ahn, Jae-Pyoung (Nano-Materials Research Center, Korea Institute of Science and Technolog) ;
  • Huh, Moo-Young (Division of Materials Science and Engineering, Korea University) ;
  • Park, Jong-Ku (Nano-Materials Research Center, Korea Institute of Science and Technology)
  • Published : 2004.06.01

Abstract

We report a carbothermal reduction process for massive synthesis of monolithic W$_{18}$O$_{49}$ phase from tungsten oxide in the presence of carbon source. Carbon black powder was used as a carbon source and added to WO$_3$ by 40 weight percent. Bundles of W$_{18}$O$_{49}$ rods were formed over the temperature range of 80$0^{\circ}C$$^{\circ}C$ to 90$0^{\circ}C$. Pure W$_{18}$O$_{49}$ bundles could be separated from the mixture of W$_{18}$O$_{49}$ and residual carbon black powder. Field emission character of W$_{18}$O$_{49}$ phase was determined using the extracted W$_{18}$O$_{49}$ rods. Flat lamp fabricated from the W$_{18}$O$_{49}$ rods showed the turn-on field of 9.3 V/${\mu}m$.

Keywords

References

  1. Solar Energt Mat. & Solar Cells. v.58 K.Bange https://doi.org/10.1016/S0927-0248(98)00196-2
  2. J. Appl. Phys. v.89 no.5 J.L.Solis;A.Hoel;V.Lantto;CG.Granqvist https://doi.org/10.1063/1.1343520
  3. Solid State Ionics v.86-88 Y.J.Li;P.P.Tsai https://doi.org/10.1016/0167-2738(96)00241-X
  4. J. Phys. Cond. Mat. v.10 A.Aird;E.K.H.Salje https://doi.org/10.1088/0953-8984/10/22/003
  5. Chem. Phys. Lett. v.309 Y.Q.Zhu;W.Hu;W.K.Hsu;M.Terrones;N.Grobert;J.P.Hare;H.W.Kroto;D.R.M.Walton;H.Terrones https://doi.org/10.1016/S0009-2614(99)00732-0
  6. Chem. Phys. Lett. v.372 Z.Liu;Y.Bando;C.Tang https://doi.org/10.1016/S0009-2614(03)00397-X
  7. Adv. Mater. v.15 no.15 Y.Li;Y.Bando;D.Golberg https://doi.org/10.1002/adma.200305122
  8. Thermochimica Acta v.282/283 D.S.Venables;M.E.Brown https://doi.org/10.1016/0040-6031(95)02814-5
  9. J. Eur. Ceram. Soc. v.20 R.Koc;S.K.Kodambaka https://doi.org/10.1016/S0955-2219(00)00038-8
  10. J. Mat. Sci. v.35 G.A.Swift;R.Koc https://doi.org/10.1023/A:1004760719005
  11. Thermochimica Acta v.291 D.S.Venables;M.E.Brown https://doi.org/10.1016/S0040-6031(96)03068-7
  12. Thermochimica Acta v.282/283 D.S.Venables;M.E.Brown https://doi.org/10.1016/0040-6031(96)02813-4
  13. Phys. Chem. Chem. Phys. v.4 T.Xiao;A.Hanif;A.P.E.York;J.Sloan;M.L.H.Green https://doi.org/10.1039/b202518c