원자력 사고후 쌀알과 배추내 $^{90}Sr$$^{137}Cs$ 농도 예측

Predictions of $^{90}Sr$ and $^{137}Cs$ Concentrations in Rice Seeds and Chinese Cabbage after a Nuclear Accident

  • 발행 : 2002.09.30

초록

원자력 사고후 시간경과에 따른 작물체내 핵종 농도를 보다 현실적으로 예측할 수 있는 방법을 수립하고 단위 건침적에 대하여 백미와 배추내 $^{90}Sr$$^{137}Cs$의 50 년간 농도를 예측하였다. 비생육기 사고의 경우 농도는 두 핵종 모두 시간경과에 따라 서서히 감소하였고 50 년 내내 $^{90}Sr$$^{137}Cs$보다 높았다. 생육기 사고의 경우 처음 1년간 농도는 비생육기 사고에 비해 대체로 $^{90}Sr$은 최고 30 배, $^{137}Cs$은 최고 1,000 배 정도까지 높았다. 50 년간의 누적농도는 백미에서는 비생육기 사고의 경우 $^{90}Sr$이, 생육기 사고의 경우 $^{137}Cs$이 더 높았으나 배추에서는 어느 경우에나 $^{90}Sr$이 더 높았다. 생육기 사고시 50 년간의 누적농도에 대한 지배적 경로는 대체로 $^{90}Sr$의 경우 뿌리흡수, $^{137}Cs$의 경우 작물체 직접오염이었다. 재부유의 영향은 무시할 수 있을 정도였다. 예측결과에 입각하여 사고 조건별로 대책의 방향을 제시하였다.

A method of more realistically, predicting radionuclide concentrations in crop plants varying with time after a nuclear accident was established to estimate 50 years' concentrations of $^{90}Sr$ and $^{137}Cs$ in polished rice seeds and Chinese cabbage for unit dry deposition. After non-growing season accidents, concentrations of both nuclides decreased gradually with time and $^{90}Sr$ concentrations were higher than those of $^{137}Cs$ throughout the whole period. Radionuclide concentrations in the 1 st year after growing season accidents were on the whole higher than those after non-growing season accidents by factors of up to 30 for $^{90}Sr$ and up to 1,000 for $^{137}Cs$. In polished rice seeds, the 50 years-integrated concentration was higher for $^{90}Sr$ than for $^{137}Cs$ after non-growing season accidents, whereas the opposite was true after growing season accidents. In Chinese cabbage. however, it was higher for $^{90}Sr$ than for $^{137}Cs$ after both types of the accident. Generally speaking, the dominant pathway for the integrated concentration after the growing season accident was root uptake for $^{90}Sr$ and direct plant contamination for $^{137}Cs$. The effect of resuspension was negligible. Based on the predicted results. the direct]on of planning countermeasures was suggested for various accident conditions.

키워드

참고문헌

  1. 이창우, 최용호, 황원태, 이정호, '쌀 섭취경로에서 동적모델을 사용한 장반감기 핵종의 거동해석 및 내부피폭선량 계산,' 대한방사선방어학회지, 17, 15-22 (1992)
  2. M. L. Abbott and A. S. Rood, 'COMIDA : a radionuclide food chain model for acute fallout deposition,' Health Physics 66, 17-29 (1994)
  3. Y. H. Choi, K. M. Lim, D. Yu, H. G. Park, Y. G. Choi and C. M. Lee, 'Transfer pathways of $^{54}Mn$, $^{57}Co$, $^{85}Sr$, $^{103}Ru$ and $^{134}Cs$ in rice and radish plants directly contaminated at different growth stages,' Annals of Nuclear Energy 29, 429-446 (2002)
  4. H. Muller and G. Prohl, 'ECOSYS-87: a dynamic model for assessing radiological consequences of nuclear accidents,' Health Physics 64, 232-252 (1993)
  5. F. W. Whicker and T. B. Kirchner, 'PATHWAY: a dynamic' food-chain model to predict radionuclide ingestion after fallout deposition,' Health Physics 52, 717-737(1987)
  6. W. T. Hwang, G. Cho and M. H. Han, 'Development of a dynamic food chain model DYNACON and its application to Korean agricultural conditions,' J. of Nuclear Science and Technology 35, 454-461 (1998)
  7. J. Ehrhardt and A. Weis (Eds), RODOS : Decision Support System for Off-Site Nuclear Emergency Management in Europe, EUR 19144 EN, Furopean Commission (2000)
  8. 이정호 등, 섭취 및 호흡에 의한 방사선 내부 피폭선량 평가 코드 개발, KAERl/RR-998/90, 한국원자력연구소 (1991)
  9. 최용호, 조재성, 이창우, 홍광희, 이정호, '벼재배기간중 침적사기에 따른 $^{54}Mn$, $^{60}Co$, $^{85}Sr$, $^{137}Cs$의 뿌리흡수,' 대한방사선방어학회지, 20, 255-263 (1995)
  10. 최용호, 조재성, 이창우, 이명호, 김상복, 홍광희, 최근식, 이정호, '주요 작물의 생육중에 침적한 $^{54}Mn$, $^{60}Co$, $^{85}Sr$, $^{137}Cs$의 지하이동,’ 대한방사선방어학회지, 21, 51-58 (1996)
  11. Y. H. Choi, C. W. Lee, S. R. Kim, J. H. Lee and J. S. Jo, 'Effect of application time of radionuclides on their root uptake by Chinese cabbage and radish,' J. of Environmental Radioactivity 39, 183-198 (1998)
  12. Y. H. Choi, K. M. Lim, H. G. Park, D. W. Park and W. Y. Lee, 'Four years' root uptake and underground distribution of $^{60}Co$ and $^{137}Cs$ in simulated rice and Chinese cabbage fields,' Proc. of IRPA10 Congress, Hiroshima, May 2000 (2000)
  13. 최용호, 임광묵, 박효국, 이원윤, 이창우, ' $^{85}Sr$, $^{103}Ru$, $^{134}Cs$의 엽면처리 시기에 따른 배추의 방사능 오염,' 대한방사선방어학회지, 23, 219-227 (1998)
  14. A. C. Chamberlain, 'Interception and retention of radioactive aerosol by vegetation,' Atmospheric Environment 4, 57-78 (1970)
  15. C. W. Miller, 'An analysis of measured values for the fraction of a radioactive aerosol intercepted by vegetation,' Health Physics 38, 705-712 (1980)
  16. 농림부, 농림수산통계연보, 31000-51023-26-01(1996)
  17. 이은웅 등, 4정 수도작, 향문사 (1996)
  18. 조성진, 박천서, 엄대익 등, 3정 토양학, 향문사 (1997)
  19. F. O. Hoffman and C. F. Baes Ill, A Statistical Analysis of Selected Parameters for Predicting Food Chain Transport and Internal Dose of Radionuclides, NUREG/CR-1004, ORNL/NUREG/TM-282, Oak Ridge National Laboratory (1979)
  20. International Atomic Energy Agency, Modelling of Resuspension, Seasonality and Losses during Food Processing, First Report of the VAMP Terrestrial Working Group, lAEA-TECDOC-647, lAEA, Vienna (1992)
  21. International Atomic Energy Agency, Generic Models and Parameters for Assessing the Environmental Transfer of Radionuclides from Routine Releases, Safety Series No. 57, IAEA, Vienna (1982)
  22. 최용호, 벼와 주요 밭작물에서 $^{54}Mn$, $^{60}Co$, $^{85}Sr$, $^{137}Cs$ 의 토양-작물계 내의 흡수, 이동 및 분포, 박사학위논문, 충남대학교 (1995)
  23. E. M. Romney, J. W. Neel, H. Nishita, J. H. Olafson and K. H. Larson, 'Plant uptake of $^{90}Sr$, $^{91}Y$, $^{106}Ru$, $^{137}Cs$ and $^{144}Ce$ from Soils,' Science 83, 369-376 (1957)
  24. H. M. Squire and L. J. Middleton, 'Behavior of $^{137}Cs$ in soils and pastures : a long-term experiment,' Radiation Botany 6, 413-425(1966)
  25. D. C. Adriano, K. W. McLeod and T. G. Ciravolo, 'Long-term 'root uptake of radiocesium by several crops,' J. of Plant Nutrition 7, 1415-1432 (1984)
  26. H. Noordijk, K. E. van Bergeijk, J. Lembrechts and M. J. Frissel, 'Impact of ageing and weather conditions on soil-to-plant transfer of radiocesium and radiostrontium,' J. of Environmental Radioactivity 15, 277-286 (1992)
  27. A. Tsumura, M. Komamura and H. Kobayashi, 'Behavior of radioactive Sr and Cs in soils and soil-plant system,' In : Report of National Institute of Agricultural Science - B, No 36, p.57-113 (in Japanese) (1983)
  28. J. E. Till and H. R. Meyer (Eds.), Radiological Assessment, NUREG/CR- 3332, ORNL-5968, U.S. Nuclear Regulatory Commission (1983)
  29. 최용호, 조재성, 이명호, 최근식, 이정호, '염화칼리와 석회의 동시살포가 주요 작물의 생육중에 침적한 $^{54}Mn$, $^{60}Co$, $^{85}Sr$, $^{137}Cs$ 의 뿌리 흡수에 미치는 영향' 대한방사선방어학회지, 20, 245-253 (1995)