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Vinylogous Intramolecular Nucleophilic Acyl Substitution Reactions Mediated by Samarium(II) Iodide


Abstract

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References

  1. Lanthanides: Chemistry and Use in Organic Synthesis Kagan, H. B.;Namy, J. L.;Kobayashi, S.(ed.)
  2. Chem. Rev. no.99 Krief, A.;Laval, A.-M.
  3. J. Org. Chem. no.59 Molander, G. A.;Shakya, S. R.
  4. J. Am. Chem. Soc. no.115 Molander, G. A.;McKie, J. A.
  5. J. Org. Chem. no.62 Molander, G. A.;Harris, C. R.
  6. The structure of the 3-(3-hydroxypropyl)cyclohex-2-one (3) was unambiguously identified by comparing it with the authentic sample which was prepared according to the method reported in the literature
  7. J. Org. Chem. no.47 Godleski, S. A.;Valpey, Rr. S.
  8. J. Org. Chem. no.47 Becker, D.;Harel, Z.; Nagler, M.; Gillon, A.
  9. J. Am. Chem. Soc. no.111 Imamoto, T.;Takiyama, N.;Nakamura, K.;Hatajima, T.;Kamija, Y.
  10. Synth. Com-mun. no.22 Crimmins, M. T.;Dedopoulou, D.
  11. Tetrahedron no.46 The spiro compound 2 was also identified by spectro-scopic method and comparing with the $^1H$ and$^{13}C$ NMR, and DEPT data with those reported in the literature. Mid-dleton D. S.;Simpkins, N. S.
  12. J. Org. Chem. no.56 Molander, G. A.;Mckie, J. A.
  13. Tetrahedron Lett. no.41 Kang, H.-Y.;Song, S.-E.
  14. Typical Procedure: 3-(3-Hydroxypropyl)cyclohex-2-enone. 3-(3-Iodopropoxy)cyclohex-2-enone (200 mg, 0.71 mmol) in THF (2.0 mL) was added dropwise to a solution of SmI2 (4.3 mmol) in THF/HMPA (10% v/v) at 0 °C under nitrogen atmosphere. After stirring for 30 min at 0 °C, the reaction mixture was quenched with Rochells salt solu-tion. $^{10}$ Extraction with dichloromethane, drying $(MgSO_4)$, and concentration followed by flash chromatography pro-vided the desired hydroxyketone as a colorless oil
  15. Synth. Commun. no.27 Schwaebe, M. K.;Little, R. D.

Cited by

  1. ChemInform Abstract: Vinylogous Intramolecular Nucleophilic Acyl Substitution Reactions Mediated by Samarium(II) Iodide. vol.32, pp.15, 2001, https://doi.org/10.1002/chin.200115065