Selective Removal of Toxic Heavy Metals in Fe-Coagulants

철염 응집제 중 유독성 중금속의 선택적 제거

  • 박상원 (계명대학교 환경과학대학)
  • Published : 1999.06.01

Abstract

Among various reactions which metal sulfides can undergo in the reducing environment, the lattice exchange reaction was examined in a attempt to selectively remove heavy metal ions contained in the Fe-Coagulants acid solution. We have examined Zeta potential along with pHs to investigate surface characteristics of ${FeS}_{(s)}$. As a result of this experiment, zero point charge(ZPC) of FeS is pH 7 and zeta potential which resulted from solid solution reaction between Pb(II) and ${FeS}_{(s)}$ is similar to that of ${PbS}_{(s)}$. Solubility characteristics of ${FeS}_{(s)}$ is appeared to that dissolved Fe(II) concentration increased in less than pH 4, and also increased with increasing heavy metal concentration. Various heavy metal ions(Pb(II), Cu(II), Zn(II)) contained in Fe-coagulants acid solution were removed selectively more than ninety-five percent in the rang of pH 2.5~10 by ${FeS}_{(s)}$. From the above experiments, therefore, We could know that the products of reaction between heavy metal ions and $FeS_{(S)}$ are mental sulfide such as $PbS_{(S)}$, $CuS_{(S)}$ and $ZnS_{(S)}$.

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References

  1. Control and treatment technology for the metal finishing industry sulfide precipitation EPA
  2. Water Research v.23 Chemical substitution reaction at the hydrous CdS surface Park, S.W.;C.P. Huang
  3. Geochim. Cosmochim. Acta v.43 Heavy metal adsorption by sulphide solutions Jean, G.E.;G.M. Bancroft
  4. J. Colloid Interface Science v.128 The adsorption characteristics of some heavy metal ions on the hydrous CdS surface Park, S.W.;C.P. Huang
  5. AICHE Symp. Ser. v.71 Adsorption of Zinc(II) at the Cinnabar (HgS)/H₂O Interface James, R.O.;G.A. Parks
  6. J. Colloid Interface Science v.117 The surface acidity of hydrous CdS Park S.W.;C.P. Huang
  7. J. Chem. v.30 adsorption of calcium at the zinc sulfide-water interface Moigmard, M.S.;R.O. James;T.W. Healy
  8. Aquatic Chemistry Stumm;J.J. Morgan
  9. Process chemistry for water and wastewater treatment Benefield, D.L.;J.F. Judkins;B.L. Weand
  10. Geochim. Cosmochim. Acta v.49 the distribution of divalent trace elements between sulfides oxides, silicates and hydrothermal solutions Sverjensky, D.A.