DOI QR코드

DOI QR Code

Application of a Novel Carbon Regeneration Process for Disposal of APEG Treatment Waste


Abstract

The chemical waste treatment, APEG (alkali/polyethylene glycol) process has been shown to be effective for the dechlorination of PCBs in transformer oil. Considerable amount of PCBs, however, still remains in the waste exceeding the 25-50 ppm limit set by regulatory agency. A new thermal regeneration technology has been developed in our laboratory for disposal of hazardous organic wastes. Due to the limited oxidation of carbon surface through the reverse movement of flame front to oxidant flow, this technology was termed counterflow oxidative system (COS). Specially, the oxidant flow in the COS process is a principal parameter which determines the optimum conditions regarding acceptable removal and destruction efficiency of adsorbed organic wastes at minimal carbon loss. The COS process, under optimum conditions, was found to be very effective and the removal and destruction efficiency of 99.99% or better was obtained for residual PCBs in the waste while bulk (≥90%) of carbon was recovered. Any toxic formation of polychlorinated dibenzo-p-dioxins (PCDDs) and polychlorinated dibenzo furans (PCDFs) were not detected in the regenerated carbon and impinger traps. The results of surface area measurement showed that the adsorptive property of regenerated carbon is mostly reclaimed during the COS process.

Keywords

References

  1. The Chenistry of PCBs Hutzinger, O.;Sage, S.;Zikto, V.
  2. Halogenated Biphenyls, Terphenyls, Naphthalenes, Dibenzofurans, and Related Products Kimbrough, R. D.
  3. Environ. Pollut. v.5 Tenabe, S.
  4. Environ. Sci. Technol. v.23 Mauchester-Neesving, J.;Andreu, A.
  5. Environ. Sci. Technol. v.24 Hermanson, M.;Hites, R.
  6. Analytical Chenistry of PCBs; Butterworth Publishers Mitchell, D. E.
  7. Process; Electric Power Research Institute (EPRI), PCB Conference Determination of Relative Efficiencies of PCB Treatment Ruggeri, B.;Kapila, S.;Camino, G.;Tumiatti, W.
  8. Treatmint Techmologies Organic Containing Waste Supernant, N.;Nunno, T.;Krawell, M.
  9. Proceedings of Dioxine 90, 10th International Meeting in Organohalogen Compounds v.2 PCB Determination Practices and Techmologies in the U. S. A. Friedman, A. J.
  10. Chemosphere v.1 Buser, H. R.;Bosshardt, H. P.;Rappe, C.
  11. Inviron, Sci. Technol. v.19 Brunelle, D. J.;Mendiratta, A. K.;Singleton, D. A.
  12. PH.D. Dissertation, University of Missouri-Rolla Ryoo, K. S.
  13. Activated Carbon Manufacture and Regeneration Yehaskel, A.
  14. Carbon v.1 no.27 Wigmans, J.
  15. Chemica Scripta v.1 Karlsson, L.;Rosen E.
  16. Environ. Sci. Technol. v.23 Schulz, D. E.;Petrick, G.;Duinker, J.