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Thermochemical Behaviour of Some Salicylaldehyde G-P Complexes of Fe(Ⅲ), Co(Ⅱ), Cu(Ⅱ) and Zn(Ⅱ)

  • Hafez, M.A.H. (Department Chemistry, Faculty of Science, Mansoura University) ;
  • Moussa, M.N.H. (Department Chemistry, Faculty of Science, Mansoura University)
  • Published : 1992.06.20

Abstract

Through two different techniques TGA and DSC the thermal decomposition processes of salicyaldehyde G-P complexes having the general formula: $$[MCl_2(L)_2]^{2+}$2Cl^-$; where L = salicyaldehyde carbohydrazone pyridinum cation, and M= Fe(III), Co(II), Cu(II) and Zn(II), have been studied. From the obtained thermogravimetric curves the following parameters n, $E_{\alpha}$, A, ${\Delta}S^{\neq}$, ${\Delta}H^{\neq}$ and ${\Delta}G^{\neq}$ were evaluated. The effect of the nature of the metal ions present in the complexes studied upon the calculated thermodynamic parameters was reported. A suitable mechanism for the thermal decomposition process was suggested.

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