DOI QR코드

DOI QR Code

Study on Separation of Heavy Metal Ions in A Neutral Macrocycle-Mediated Emulsion Liquid Membrane System

  • Moon-Hwan Cho (Institute of Basic Science and Department of Chemistry, Kang Weon National University) ;
  • Hea-Suk Chun (Institute of Basic Science and Department of Chemistry, Kang Weon National University) ;
  • Jin-Ho Kim (Institute of Basic Science and Department of Chemistry, Kang Weon National University) ;
  • Chang-Hwan Rhee (Institute of Basic Science and Department of Chemistry, Kang Weon National University) ;
  • Si-Joong Kim (Department of Chemistry, Korea University)
  • Published : 1991.10.20

Abstract

The preferential transport phenomena of neutral cation-anion moieties in neutral macrocycle-facilitated emulsion liquid membrane were described in this study. Emulsion membrane systems consisting of (1) aqueous source phase containing 0.001 M M($NO_3$)$_2(M=Mn^{2+},\;Co^{2+},\;Ni^{2+},\;Cu^{2+},\;Zn^{2+},\;Sr^{2+},\;Cd^{2+},\;and\;Pb^{2+})$ (2) a toluene membrane containing 0.01 M ligand $(DBN_3O_2$, DA18C6, DT18C6, TT18C6, HT18C6) and the surfactant span 80 (sorbitan monooleate) (3% v/v) and (3) an aqueous receiving phase containing $Na_2S_2O_3$ or $NaNO_3$ were studied with respect to the disappearence of transition metal ions from the source phase as a function of time. Cation transports for various two component or three component equimolar mixture of transition metal and $Cu^{2+}$ in a emulsion membrane system incorporating macrocyclic ligand (HT18C6) as carrier were determinded. $Cu^{2+}$ was transported higher rates than the other $M^{2+}$ in the mixture solution. Equilibrium constants for cation-source phase co-anion, cation macrocycle and cation-receiving phase reagent interaction are examined as parameters for the prediction of cation transport selectivities.

Keywords

References

  1. J. Am. Chem. Soc. v.107 J. P. Behr;J. M. Lehn
  2. J. Membr. Sci. v.10 H. K. Lonsdale
  3. J. Membr. Sci. v.12 J. D. Way;R. D. Noble;T. M. Flynn;E. D. Sloan
  4. Bull. Korean Chem. Soc. v.9 M. H. Cho;K. H. Seon-Woo;S. J. Kim
  5. Sep. Sci. and Tech. v.5 F. Nakashio;K. Kondo
  6. J. Membr. Sci. v.2 R. W. Baker;M. E. Tuttle;D. J. Kelly;H. K. Lonsdale
  7. Ind. Eng. Chem., Process Des. Dev. v.10 N. N. Li
  8. J. Membr. Sci. v.24 R. M. Izatt;G. A. Clark;J. J. Christensen
  9. J. Memb. Sci. v.33 R. M. Izatt;M. H. Cho
  10. Anal. Chem. v.59 R. M. Izatt;M. H. Cho;J. D. Lamb;J. J. Christensen

Cited by

  1. Ion Flotation of Zinc(II) and Cadmium(II) in the Presence of Side-Armed Diphosphaza-16-Crown-6 Ethers vol.38, pp.3, 1991, https://doi.org/10.1081/ss-120016655
  2. Pyrrole Azocrown Ethers. Synthesis, Complexation, Selective Lead Transport and Ion-Selective Membrane Electrode Studies vol.18, pp.7, 1991, https://doi.org/10.1080/10610270600879068
  3. Supported Liquid (SLM) and Polymer Inclusion (PIM) Membranes Pertraction of Copper(II) from Aqueous Nitrate Solutions by 1-Hexyl-2-Methylimidazole vol.47, pp.9, 2012, https://doi.org/10.1080/01496395.2012.672523