Some Physical and Chemical Properties of Synthesized Dawsonite

합성 Dawsonite의 물리적, 화학적 성질

  • 권상욱 (한양대학교 문리과대학)
  • Published : 19690600

Abstract

$NaAl(OH)_2CO_3$was synthesized using colloidal earth (Allophane) as the starting material and some of its were studied in detail. It was found that Dawsonite was formed in the pH range (pH 12.5~12.0) that the concentration of $HCO_3^-$ was just begun to increase and the presence of $HCO_3^-$ in the product was clarified from the infrared absorption spectrum. The chemical formular of Dawsonite was therefore presumed as $NaAlO (OH) HCO_3$. From toahhe results of X-ray powder diffraction, both peaks at 5.7 $\AA$ and 2.8 $\AA$ were observed, and fibrous crystalline structure was observed from electron micrograph and also found from the microscopic electron diffraction at 5.7 $\AA.$ Therefore the fibrous axis was considered as =Al=O2=Al=O2=Al=(*image) direction. True specific gravity of Dawsonite was 2.44 and its porosity was 91.4%. It was practically insoluble in water, but decomposed in the boiling water to form Pseudo Boehmite. Stable pH range of Dawsonite was about 4.5~11.5. From the results of D.T.A. and T.G.A., it was observed that $CO_2$was liberated at $350^{\circ}C$, and $H_2O$ at $650^{\circ}C$, and converted into strongly hygroscopic $NaAlO_2$, which was easily decomposed in water into $\beta-Al(OH)_3(Bayerite)$ and NaOH.

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References

  1. Tonerde und Aluminium v.I W.Fulda;H. Ginsberg
  2. 早稻田應化誌 v.21 田中;海野
  3. Bullentin of Sci Eng. v.41 Sang Wook;Kwon;Ishikawa
  4. 日本粘土學會討論會講演要旨
  5. Accad, Ital v.3 no.7 Richerche roentgen grofiche sulla Dawsonite, prima resalati Sperimentali R. C. Lauro;Carlo
  6. ASTM card 12-449
  7. Anal, chem v.26 L.D. Frederickson
  8. 鑛物學名辭典 木下龜城
  9. ASTM card 2-0985
  10. ASTM card 13-15
  11. J. phys. chem. v.38 H.B. weisar
  12. ASTM card 12-457
  13. U. Allgem. Chem. v.175 R. Fricke;Z. Aanorg
  14. U. Allgem. Chem. v.179 R. Fricke;Z. Aanorg
  15. 日本工化誌 v.55 舟木好右衛;內材孝太郞
  16. Infrared Spectra of Inorganic and coordination compounds K. Nakamoto
  17. Anal, Chem. v.24 F.A. Miller;C.H. Wilkins
  18. Synthesized dawsonite, Bulletin of Sci. v.41 Sang Wook;Kwon;Ishikawa