Syntheses of Metallic Monoazo Complexes

Monoazo 金屬錯염의 合成

  • Published : 19680900

Abstract

Some ortho-hydroxy monoazo-compounds have been synthesized and these were metallized with transition elements. Chromium trioxide, cupric acetate and cobalt acetate were used for the metallization. The following facts have been found in this investigation: (1) water is the best solvent, when compared to various organic solvents, for the metallization, (2) the optimum pH for the metallizing mixture ranges from 4.5 to 5.5, (3) the solubility of these metallic monoazo-compounds in water depends mainly on the composition of the complexes and to some extent on the presence of sulfonic acid groups in the molecules, and (4) metallized compounds having two ortho-hydroxy groups per molecule have stronger binding characteristics.

몇가지 ortho-hydroxy monoazo 化合物들을 合成하여 이것들을 遷移元素로 金屬化시켰다. 三酸化크롬, 酢酸銅 및 酢酸코발드를 이 金屬錯鹽生成反應에 使用하였다. 이 硏究에서 다음과 같은 事實들을 알 수 있었다. (1) 이 金屬錯鹽生成反應에서의 溶媒는 다른 여러가지 有機溶媒보다는 물이 가장 좋고, (2) 金屬錯鹽生成反應 混合液의 가장 適當한 液性은 pH=4.5~5.5程度 이었으며, (3) 이들 monoazo 金屬錯鹽의 물에 대한 溶解性은 主로 그 錯鹽의 組成에 달렸으나 어느 程度는 分子內의 黃酸基의 存在에 의하여서도 影響을 받는다. 그리고 (4) 分子當 두개의 ortho-hydroxy基를 가진 金屬錯鹽이 더 强한 結合能을 가지고 있다.

Keywords

References

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