The Complexes of Fluorobenzene with Halogens and Interhalogens in Carbon Tetrachloride

플루오로벤젠과 할로겐 또는 할로겐間化合物 사이의 錯物에 관한 연구

  • Published : 19670900

Abstract

The interactions of fluorobenzene with iodine monochloride, iodine monobromide, bromine and chlorine in carbon tetrachloride solution have been examined through ultraviolet spectrophotometric measurements. The results indicate the formation of one to one molecular complexes, $C_6H_5F{\cdot}ICl$, $C_6H_5F{\cdot}IBr$, $C_6H_5F{\cdot}Br_2$, and $C_6H_5F{\cdot}Cl_2$ in solution. The equilibrium constants obtained at room temperature for the formation of these four complexes are 0.161, 0.072, 0.045 and 0.035 l $mole^{-1}$, respectively. Comparison of these results with those reported in the literature on other complexes of similar type reveals that the relative stabilities of these complexes decrease in the following orders: ICl>IBr>$I_2$>$Br_2$>$Cl_2$ $C_6H_6$>$C_6H_5Br$>$C_6H_5Cl$>$C_6H_5F$

플루오르벤젠과 일염화요오드, 일브롬화요오드, 브롬 또는 염소의 각 系를 사염화탄소 용액에서 分光光度法에 의하여 연구한 결과, $C_6H_5F{\cdot}ICl$, $C_6H_5F{\cdot}IBr$, $C_6H_5F{\cdot}Br_2$, 또는 $C_6H_5F{\cdot}Cl_2$의 錯物이 형성됨을 알았다. 이들 錯物형성에 대한 실온에서의 평형상수는 각각 0.161, 0.072, 0.045 및 0.035 l $mole^{-1}$이다. 이 결과와 문헌에 보고된 연구결과를 종합적으로써 이러한 착물의 상대적 안정도가 다음 순으로 감소함을 알 수 있었다. ICl>IBr>$I_2$>$Br_2$>$Cl_2$ $C_6H_6$>$C_6H_5Br$>$C_6H_5Cl$>$C_6H_5F$

Keywords

References

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