Preparation of Pt impregnated Nafion self-humidifying membranes for PEMFC using supercritical $CO_2$

초임계 함침법을 이용한 PEMFC용 Pt/Nafion 자가가습막의 제조 연구

  • Published : 2006.11.23

Abstract

Pt/Nafion self-humidifying membranes for Polymer Electrolyte Membrane Fuel Cell(PEMFC) were synthesized via supercritical-impregnation methods. The Nafion 112 membranes were impregnated with Pt(II)$(acetylacetonate)_2$ from a supercritical carbon dioxide $(scCO_2)$ solution at $80^{\circ}C$ and 30MPa. After the impregnation, the pressure decreased slowly by releasing $CO_2$. And the Pt-impregnated Nafion membrane was converted Pt deposited Nafion membrane by reducing agent, sodium borohydride $(NaBH_4)$ with various concentrations under $50^{\circ}C$ and 2 hours. The prepared Pt-impregnated Nafion (Pt/Nafion) composite membrane were investigated by Electron Prove Micro analysis (EPMA) and X-rat Diffraction analysis (XRD) which showed distribution of Pt particle and Scanning Electron Microscopy (SEM) and Atomic Force Microscopy (AFM) a which revealed morphology of surface of Pt/Nafion composite membrane. The performance of the Pt/Nafion 112 membranes was examined in PEMFC as aself-humidifyin membranes using purpose-built equipment.

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